Referierte Publikationen

In this study, we propose two full-optical-setup and single-shot measurable approaches for complete characterization of attosecond pulses from surface high harmonic generation (SHHG): SHHG-SPIDER (spectral phase interferometry for direct electric field reconstruction) and SHHG-SEA-SPIDER (spatially encoded arrangement for SPIDER). 1D- and 2D-EPOCH PIC (particle-in-cell) simulations were performed to generate the attosecond pulses from relativistic plasmas under different conditions. Pulse trains dominated by single isolated peak as well as complex pulse train structures are extensively discussed for both methods, which showed excellent accuracy in the complete reconstruction of the attosecond field with respect to the direct Fourier transformed result. Kirchhoff integral theorem has been used for the near-to-far-field transformation. This far-field propagation method allows us to relate these results to potential experimental implementations of the scheme. The impact of comprehensive experimental parameters for both apparatus, such as spectral shear, spatial shear, cross-angle, time delay, and intensity ratio between the two replicas has been investigated thoroughly. These methods are applicable to complete characterization for SHHG attosecond pulses driven by a few to hundreds of terawatts femtosecond laser systems.

Measuring signatures of strong-field quantum electrodynamics (SF-QED) processes in an intense laser field is an experimental challenge: it requires detectors to be highly sensitive to single electrons and positrons in the presence of the typically very strong x-ray and gamma-photon background levels. In this paper, we describe a particle detector capable of diagnosing single leptons from SF-QED interactions and discuss the background level simulations for the upcoming Experiment-320 at FACET-II (SLAC National Accelerator Laboratory). The single particle detection system described here combines pixelated scintillation LYSO screens and a Cherenkov calorimeter. We detail the performance of the system using simulations and a calibration of the Cherenkov detector at the ELBE accelerator. Single 3 GeV leptons are expected to produce approximately 537 detectable photons in a single calorimeter channel. This signal is compared to Monte-Carlo simulations of the experiment. A signal-to-noise ratio of 18 in a single Cherenkov calorimeter detector is expected and a spectral resolution of 2% is achieved using the pixelated LYSO screens.

The Free-Electron Laser (FEL) FLASH offers the worldwide still unique capability to study ultrafast processes with high-flux, high-repetition rate extreme ultraviolet, and soft X-ray pulses. The vast majority of experiments at FLASH are of pump-probe type. Many of them rely on optical ultrafast lasers. Here, a novel FEL facility laser is reported which combines high average power output from Yb:YAG amplifiers with spectral broadening in a Herriott-type multipass cell and subsequent pulse compression to sub-100-fs durations. Compared to other facility lasers employing optical parametric amplification, the new system comes with significantly improved noise figures, compactness, simplicity, and power efficiency. Like FLASH, the optical laser operates with 10-Hz burst repetition rate. The bursts consist of 800-mu s long trains of up to 800 ultrashort pulses being synchronized to the FEL with femtosecond precision. In the experimental chamber, pulses with up to 50-mu J energy, 60-fs full-width half-maximum duration and 1-MHz rate at 1.03-mu m wavelength are available and can be adjusted by computer-control. Moreover, nonlinear polarization rotation is implemented to improve laser pulse contrast. First cross-correlation measurements with the FEL at the plane-grating monochromator photon beamline are demonstrated, exhibiting the suitability of the laser for user experiments at FLASH.

High-resolution Fourier-transform spectroscopy using table-top sources in the extreme ultraviolet (XUV) spectral range is still in its infancy. In this contribution a significant advance is presented based on a Michelson-type all-reflective split-and-delay autocorrelator operating in a quasi amplitude splitting mode. The autocorrelator works under a grazing incidence angle in a broad spectral range (10 nm - 1 µ m) providing collinear propagation of both pulse replicas and thus a constant phase difference across the beam profile. The compact instrument allows for XUV pulse autocorrelation measurements in the time domain with a single-digit attosecond precision resulting in a resolution of E/Δ E=2000. Its performance for spectroscopic applications is demonstrated by characterizing a very sharp electronic transition at 26.6 eV in Ar gas induced by the 11th harmonic of a frequency-doubled Yb-fiber laser leading to the characteristic 3s3p⁶4p¹P¹ Fano-resonance of Ar atoms. We benchmark our time-domain interferometry results with a high-resolution XUV grating spectrometer and find an excellent agreement. The common-path interferometer opens up new opportunities for short-wavelength femtosecond and attosecond pulse metrology and dynamic studies on extreme time scales in various research fields.

Off-axis parabolic telescopes are rarely used in high-intensity, high-energy lasers, despite their favorable properties for beam transport such as achromatism, low aberrations and the ability to handle high peak intensities. One of the major reasons for this is the alignment procedure which is commonly viewed as complicated and time consuming. In this article, we revisit off-axis parabolic telescopes in the context of beam transport in high-intensity laser systems and present a corresponding analytical model. Based on that, we propose a suitable setup that enables fast and repeatable alignment for everyday operation.

In atomic structure and collision theory, the efficient spin-angular integration is known to be crucial and often decides, how accurate the properties and behavior of atoms can be predicted numerically. Various methods have been developed in the past to keep the computation (and implementation) of the spin-angular integration feasible for complex shell structures, including open d- and f-shell elements. To support such computations, we here provide a new implementation of the angular coefficients for jjcoupled and symmetry-adapted configuration states that is entirely built upon the quasi-spin formalism. The moduleSpinAngularis based on Julia, a new programming language for scientific computing, and supports a simple access to all (completely) reduced tensors, coefficients of fractional parentage for subshells with j <= 9/2 as well as the re-coupling coefficients from this formalism. Moreover, this module has been worked out for multiple purposes, including 1) the accurate calculation of atomic properties, 2) further studies on spin-angular integration theory, 3) the development of new or existing computer programs as well as 4) the manipulation of reduced matrix elements from this theory. The present implementation will therefore help advance the algebraic evaluation of many-electron (transition) amplitudes and to apply the theory to newly emerging research areas.

In this work we present a novel way to manipulate the effect of transverse mode instability by inducing traveling waves in a high-power fiber system. What sets this technique apart is the fact that it allows controlling the direction of the modal energy flow, for the first time to the best of our knowledge. Thus, using the method proposed in this work it will be possible to transfer energy from the higher-order mode into the fundamental mode of the fiber, which mitigates the effect of transverse mode instability, but also to transfer energy from the fundamental mode into the higher-order mode. Our simulations indicate that this approach will work both below and above the threshold of transverse mode instability. In fact, our model reveals that it can be used to force a nearly pure fundamental mode output in the fiber laser system almost independently of the input coupling conditions. In this context, this technique represents the first attempt to exploit the physics behind the effect of transverse mode instability to increase the performance of fiber laser systems.

We investigate the delocalization of quantum information in the nonequilibrium dynamics of the XY spin chain with asymptotically decaying interactions similar to 1/r(alpha). As a figure of merit, we employ the tripartite mutual information (TMI), the sign of which indicates if quantum information is predominantly shared globally. Interestingly, the sign of the TMI distinguishes regimes of the exponent a that are known for different behaviors of information propagation. While an effective causal region bounds the propagation of information, if interactions decay sufficiently fast, this information is mainly delocalized, which leads to the necessity of global measurements. Furthermore, the results indicate that mutual information is monogamous for all possible partitionings in this case, implying that quantum entanglement is the dominant correlation. If interactions decay sufficiently slow, though information can propagate (quasi-)instantaneously, it is mainly accessible by local measurements at early times. Furthermore, it takes some finite time until correlations start to become monogamous, which suggests that entanglement is not the dominant correlation at early times. Our findings give new insights into the dynamics and structure of quantum information in many-body systems with long-range interactions, and might get verified on state-of-the-art experimental platforms.

We present a high-power source of broadband terahertz (THz) radiation covering the whole THz spectral region (0.1-30 THz). The two-color gas plasma generation process is driven by a state-of-the-art ytterbium fiber chirped pulse amplification system based on coherent combination of 16 rod-type amplifiers. Prior to the THz generation, the pulses are spectrally broadened in a multipass cell and compressed to 37 fs with a pulse energy of 1.3 mJ at a repetition rate of 500 kHz. A gas-jet scheme has been employed for the THz generation, increasing the efficiency of the process to 0.1%. The air-biased coherent detection scheme is implemented to characterize the full bandwidth of the generated radiation. A THz average power of 640 mW is generated, which is the highest THz average power achieved to date. This makes this source suitable for a variety of applications, e.g., spectroscopy of strongly absorbing samples or driving nonlinear effects for the studies of material properties.

We employed N-benzyl-2-methyl-4-nitroaniline (BNA) crystals bonded on substrates of different thermal conductivity to generate THz radiation by pumping with 800 nm laser pulses. Crystals bonded on sapphire substrate provided four times more THz yield than glass substrate. A pyrodetector and a single-shot electro-optic (EO) diagnostic were employed for measuring the energy and temporal characterisation of the THz pulse. Systematic studies were carried out for the selection of a suitable EO crystal, which allowed accurate determination of the emitted THz spectrum from both substrates. Subsequently, the THz source and single-shot electro-optic detection scheme were employed to measure the complex refractive index of window materials in the THz range.

We experimentally investigated the accelerated proton beam characteristics such as maximum energy and number by varying the incident laser parameters. For this purpose, we varied the laser energy, focal spot size, polarization, and pulse duration. The proton spectra were recorded using a single-shot Thomson parabola spectrometer equipped with a microchannel plate and a high-resolution charge-coupled device with a wide detection range from a few tens of keV to several MeV. The outcome of the experimental findings is discussed in detail and compared to other theoretical works.

The interaction of light with the quantum-vacuum is predicted to give rise to some of the most fundamental and exotic processes in modern physics, which remain untested in the laboratory to date. Electron-positron pair production from a pure vacuum target, which has yet to be observed experimentally, is possibly the most iconic. The advent of ultra-intense lasers and laser accelerated GeV electron beams provide an ideal platform for the experimental realisation. Collisions of high energy gamma-ray photons derived from the GeV electrons and intense laser fields result in detectable pair production rates at field strengths that approach and exceed the Schwinger limit in the centre-of-momentum frame. A detailed experiment has been designed to be implemented at the ATLAS laser at the centre of advanced laser applications. We show full calculations of the expected backgrounds and beam parameters which suggest that single pair events can be reliably generated and detected.

In-volume ultrafast laser direct writing of silicon is generally limited by strong nonlinear propagation effects preventing the production of modifications. By using advantageous spectral, temporal, and spatial conditions, we demonstrate that modifications can be repeatably produced inside silicon. Our approach relies on irradiation at approximate to 2 mu m wavelength with temporally distorted femtosecond pulses. These pulses are focused in a way that spherical aberrations of different origins mutually balance, as predicted by point spread function analyses and in good agreement with nonlinear propagation simulations. We also establish the laws governing modification growth on a pulse-to-pulse basis, which allows us to demonstrate transverse inscription inside silicon with various line morphologies depending on the irradiation conditions. We finally show that the production of single-pulse repeatable modifications is a necessary condition for reliable transverse inscription inside silicon.

We study the nonlinear QED signature of x-ray vacuum diffraction in the head-on collision of optical high-intensity and x-ray free-electron laser pulses at finite spatiotemporal offsets between the laser foci. The high-intensity laser driven scattering of signal photons outside the forward cone of the x-ray probe constitutes a prospective experimental signature of quantum vacuum nonlinearity. Resorting to a simplified phenomenological ad hoc model, it was recently argued that the angular distribution of the signal in the far-field is sensitive to the wavefront curvature of the probe beam in the interaction region with the high-intensity pump. In this work, we model both the pump and probe fields as pulsed paraxial Gaussian beams and reanalyze this effect from first principles. We focus on vacuum diffraction both as an individual signature of quantum vacuum nonlinearity and as a potential means to improve the signal-to-background separation in vacuum birefringence experiments.