Referierte Publikationen

We investigate the deexcitation of the 229Th nucleus via the excitation of an electron. Detailed calculations are performed for the enhancement of the nuclear decay width due to the so called electron bridge (EB) compared to the direct photoemission from the nucleus. The results are obtained for triply ionized thorium by using a B-spline pseudo basis approach to solve the Dirac equation for a local xα potential. This approach allows for an approximation of the full electron propagator including the positive and negative continuum. We show that the contribution of continua slightly increases the enhancement compared to a propagator calculated by a direct summation over bound states. Moreover we put special emphasis on the interference between the direct and exchange Feynman diagrams that can have a strong influence on the enhancement.

The contribution of the third order in magnetic field to the Zeeman splitting of the ground state of hydrogenlike, lithiumlike, and boronlike ions in the range Z=6-82 is investigated within the relativistic approach. Both perturbative and non-perturbative methods of calculation are employed and found to be in agreement. For lithiumlike and boronlike ions the interelectronic-interaction effects are taken into account within the approximation of the local screening potential. The contribution of the third-order effect in low- and medium-Z boronlike ions is found to be important for anticipated high-precision measurements.

Attosecond time-resolved photoemission spectroscopy reveals that photoemission from solids is not yet fully understood. The relative emission delays between four photoemission channels measured for the van der Waals crystal tungsten diselenide (WSe2) can only be explained by accounting for both propagation and intra-atomic delays. The intra-atomic delay depends on the angular momentum of the initial localized state and is determined by intra-atomic interactions. For the studied case of WSe2, the photoemission events are time ordered with rising initial-state angular momentum. Including intra-atomic electron-electron interaction and angular momentum of the initial localized state yields excellent agreement between theory and experiment. This has required a revision of existing models for solid-state photoemission, and thus, attosecond time-resolved photoemission from solids provides important benchmarks for improved future photoemission models.

This paper is devoted to an investigation of nonlinearly charged dilatonic black holes in the context of gravity's rainbow with two cases: (1) by considering the usual entropy, (2) in the presence of first order logarithmic correction of the entropy. First, exact black hole solutions of dilatonic Born—Infeld gravity with an energy dependent Liouville-type potential are obtained. Then, thermodynamic properties of the mentioned cases are studied, separately. It will be shown that although mass, entropy and the heat capacity are modified due to the presence of a first order correction, the temperature remains independent of it. Furthermore, it will be shown that divergences of the heat capacity, hence phase transition points are also independent of a first order correction, whereas the stability conditions are highly sensitive to variation of the correction parameter. Except for the effects of a first order correction, we will also present a limit on the values of the dilatonic parameter and show that it is possible to recognize AdS and dS thermodynamical behaviors for two specific branches of the dilatonic parameter. In addition, the effects of nonlinear electromagnetic field and energy functions on the thermodynamical behavior of the solutions will be highlighted and dependency of critical behavior, on these generalizations will be investigated.

The interaction of micro- and nano-structured target surfaces with high-power laser pulses is being widely investigated for its unprecedented absorption efficiency. We have developed vertically aligned metallic micro-pillar arrays for laser-driven proton acceleration experiments. We demonstrate that such targets help strengthen interaction mechanisms when irradiated with high-energy-class laser pulses of intensities ~10^17–18 W/cm2. In comparison with standard planar targets, we witness strongly enhanced hot-electron production and proton acceleration both in terms of maximum energies and particle numbers. Supporting our experimental results, two-dimensional particle-in-cell simulations show an increase in laser energy conversion into hot electrons, leading to stronger acceleration fields. This opens a window of opportunity for further improvements of laser-driven ion acceleration systems.

The influence of plasma environment on the atomic parameters associated with the K-vacancy states has been investigated theoretically for several iron ions. To do this, a time-averaged Debye–Hückel potential for both the electron–nucleus and electron–electron interactions has been considered in the framework of relativistic multiconfiguration Dirac–Fock computations. More particularly, the plasma screening effects on ionization potentials, K-thresholds, transition energies, and radiative rates have been estimated in the astrophysical context of accretion disks around black holes. In the present paper, we describe the behaviour of those atomic parameters for Ne-, Na-, Ar-, and K-like iron ions.

We report large-scale multi-configuration Dirac–Hartree–Fock calculations and relativistic configuration interaction calculations for allowed E1 and forbidden transitions (M1, E2, M2) among the fine structure levels of the 3s^2 3p^5, 3s 3p^6 and 3s^2 3p^4 3d configurations for Ni xii. In our systematically enlarged wave functions, we incorporated the effects of relativity, all important electron correlations and rearrangement of the bound electron density within two different computational models. We compare our calculated energies for the fine structure levels with previous calculations and experiments. We validate all the tentative experimental lines recently identified by Del Zanna & Badnell with one exception. We discuss the consistency of our transition rates in comparison to semi-empirical predictions. We present ab initio lifetime values by taking into account all allowed E1 and forbidden transitions (M1, E2, M2) rates among lowest 31 levels. Our results for lifetime values are better than previously reported ab initio and semi-empirical values as compared to available experiments, thus, providing reliable predictions in the prospects of future experiments.

We report on a theoretical and experimental study of the energy transfer between an optical evanescent wave, propagating in vacuum along the planar boundary of a dielectric material, and a beam of sub-relativistic electrons. The evanescent wave is excited via total internal reflection in the dielectric by an infrared (λ = 2 μm) femtosecond laser pulse. By matching the electron propagation velocity to the phase velocity of the evanescent wave, energy modulation of the electron beam is achieved. A maximum energy gain of 800 eV is observed, corresponding to the absorption of more than 1000 photons by one electron. The maximum observed acceleration gradient is 19 ± 2 MeV/m. The striking advantage of this scheme is that a structuring of the acceleration element’s surface is not required, enabling the use of materials with high laser damage thresholds that are difficult to nano-structure, such as SiC, Al2O3 or CaF2.

The detailed temporal evolution of the laser-wakefield acceleration process with controlled injection, producing reproducible high-quality electron bunches, has been investigated. The localized injection of electrons into the wakefield has been realized in a simple way - called shock-front injection - utilizing a sharp drop in plasma density. Both experimental and numerical results reveal the electron injection and acceleration process as well as the electron bunch's temporal properties. The possibility to visualize the plasma wave gives invaluable spatially resolved information about the local background electron density, which in turn allows for an efficient suppression of electron self-injection before the controlled process of injection at the sharp density jump. Upper limits for the electron bunch duration of 6.6 fs FWHM, or 2.8 fs (r.m.s.) were found. These results indicate that shock-front injection not only provides stable and tunable, but also few-femtosecond short electron pulses for applications such as ultrashort radiation sources, time-resolved electron diffraction or for the seeding of further acceleration stages.

High-precision QED calculations of ground-state ionization energies are performed for all boronlike ions with nuclear charge numbers in the range 16≤Z≤96. Rigorous QED calculations are performed within the extended Furry picture and include all many-electron QED effects up to the second order of the perturbation theory. The contributions of third- and higher-order electron-correlation effects are accounted for within the Breit approximation. Nuclear recoil and nuclear polarization effects are taken into account as well. In comparison with previous evaluations of the ground-state ionization energies of boronlike ions the accuracy of the theoretical predictions is improved significantly.

Laser beams with Laguerre–Gaussian (LG) mode carry orbital angular momentum (OAM); however, when interacting with plasmas, the net angular momentum acquired by plasmas is basically zero after interaction. Here, we find when there exists a small magetostatic seed along the laser propagation direction, the barrier would be broken, giving rise to dramatic angular momentum transfer from LG-lasers to plasmas. Hence, the net OAM remaining in the plasmas system would continuously enhance the magetostatic field, until the corresponding Larmor frequency of electrons is comparable to the laser frequency in vacuum. Three-dimensional particle-in-cell simulations are performed to confirm our theory, producing spatial-uniform, temporal-stable and extremely-intense magetostatic fields.

Extreme ultraviolet microscopy is technologically demanding and thus largely confined to synchrotron radiation facilities. However, specific benefits like high resolution and exceptional material contrast provide strong motivation for the development of table-top alternatives. We report on the first demonstration of coherence tomography, i.e., noninvasive cross-sectional imaging, with high harmonics. A depth resolution of 24 nm and very good material contrast are achieved. Excessively demanding optics for extreme ultraviolet radiation are avoided and artifacts due to the elementary geometry are suppressed with a novel three-step one-dimensional phase-retrieval algorithm. The images are recorded in reflection geometry, facilitating the analysis of, e.g., operating semiconductor samples.

In a recent experiment, Schmiegelow et al. [Nat. Commun. 7, 12998 (2016)] investigated the magnetic sublevel population of Ca^+ ions in a Laguerre-Gaussian light beam if the target atoms were just centered along the beam axis. They demonstrated in this experiment that the sublevel population of the excited atoms is uniquely defined by the projection of the orbital angular momentum of the incident light. However, little attention has been paid so far to the question of how the magnetic sublevels are populated when atoms are displaced from the beam axis by some impact parameter b. Here, we analyze this sublevel population for different atomic impact parameters in first-order perturbation theory and by making use of the density-matrix formalism. Detailed calculations are performed especially for the 4s ^2S_1/2 -> 3d ^2D_5/2 transition in Ca^+ ions and for the vector potential of a Laguerre-Gaussian beam in Coulomb gauge. It is shown that the magnetic sublevel population of the excited ^2D_5/2 level varies significantly with the impact parameter and is sensitive to the polarization, the radial index, as well as the orbital angular momentum of the incident light beam.

The acceleration of ions from ultrathin (10–100 nm) carbon foils has been investigated using intense (∼6×10²⁰ W cm⁻²) ultrashort (45 fs) laser pulses, highlighting a strong dependence of the ion beam parameters on the laser polarization, with circularly polarized (CP) pulses producing the highest energies for both protons and carbons (25−30  MeV/nucleon); in particular, carbon ion energies obtained employing CP pulses were significantly higher (∼2.5 times) than for irradiations employing linearly polarized pulses. Particle-in-cell simulations indicate that radiation pressure acceleration becomes the dominant mechanism for the thinnest targets and CP pulses.

An angle-resolved x-ray spectroscopic scheme is presented for determining the hyperfine splitting of highly charged ions. For heliumlike ions, in particular, we propose to measure either the angular distribution or polarization of the 1s2p ^3P_1,F -> 1s^2 ^1S_0,F_f emission following the stimulated decay of the initial 1s 2s ^1S_0,F_i level. It is found that both the angular and polarization characteristics of the emitted x-ray photons strongly depend on the (relative) splitting of the partially overlapping hyperfine 1s 2p ^3P_1,F resonances and may thus help resolve their hyperfine structure. The proposed scheme is feasible with present-day photon detectors and allows a measurement of the hyperfine splitting of heliumlike ions with a relative accuracy of about 10^-4.

Formation of triply ionized states upon the creation of 4d inner-shell holes in atomic Hg is investigated by using synchrotron radiation of 730 eV photon energy and a versatile multielectron coincidence detection technique in combination with multiconfiguration Dirac-Fock calculations. By carefully selecting Coster-Kronig electrons detected only in coincidence with a 4d photoelectron, the Coster-Kronig spectrum has been extracted and the corresponding branching ratios of the 4d hole have been determined. The results are found to differ from previously established experimental ratios based on electron impact ionization but to agree now better with theory. We also present an Auger cascade analysis of pathways leading to triply ionized states of atomic Hg upon removal of a 4d inner-shell electron.

Ultra-short laser pulses with only a few optical cycles duration have gained increasing importance during the recent decade and are currently employed in many laboratories worldwide. In addition, modern laser technology nowadays can provide few-cycle pulses at very high average power which advances established studies and opens exciting novel research opportunities. In this paper, the two complementary approaches for providing few-cycle pulses at high average power, namely optical parametric amplification and nonlinear pulse compression, are reviewed and compared. In addition, their limitations and future scaling potential are discussed. Furthermore, selected applications particularly taking advantage of the high average power and high repetition rate are presented.

We present an ultrafast fiber laser system delivering 4.6 W average power at 258 nm based on two-stage fourth-harmonic generation in beta barium borate (BBO). The beam quality is close to being diffraction limited with an M^2 value of 1.3×1.6. The pulse duration is 150 fs, which, potentially, is compressible down to 40 fs. A plain BBO and a sapphire-BBO compound are compared with respect to the achievable beam quality in the conversion process. This laser is applicable in scientific and industrial fields. Further scaling to higher average power is discussed.

Asymptotically free renormalization group trajectories can be constructed in non-Abelian Higgs models with the aid of generalized boundary conditions imposed on the renormalized action. We detail this construction within the languages of simple low-order perturbation theory, effective field theory, as well as modern functional renormalization group equations. We construct a family of explicit scaling solutions using a controlled weak-coupling expansion in the ultraviolet, and obtain a standard Wilsonian renormalization group relevance classification of perturbations about scaling solutions. We obtain global information about the quasifixed function for the scalar potential by means of analytic asymptotic expansions and numerical shooting methods. Further analytical evidence for such asymptotically free theories is provided in the large-N limit. We estimate the long-range properties of these theories and identify initial/boundary conditions giving rise to a conventional Higgs phase.

Photoelectron angular distributions following the nonresonant two-photon K-shell ionization of neutral atoms are studied theoretically. Using the independent particle approximation and relativistic second-order perturbation theory, the contributions of screening and relativistic effects to the photoelectron angular distribution are evaluated. A simple nonrelativistic expression is presented for the angle-differential cross section in dipole approximation for two-photon ionization by elliptically polarized photons, and its limitations are analyzed numerically. Moreover, we show that screening effects of the inactive electrons can significantly affect the photoelectron distributions and can also lead to a strong elliptical dichroism. Numerical results are presented for the case of two-photon K-shell ionization of neutral Ne, Ge, Xe, and U atoms.

Coherent diffraction imaging (CDI) in the extreme ultraviolet has become an important tool for nanoscale investigations. Laser-driven high harmonic generation (HHG) sources allow for lab scale applications such as cancer cell classification and phase-resolved surface studies. HHG sources exhibit excellent coherence but limited photon flux due poor conversion efficiency. In contrast, table-top soft X-ray lasers (SXRL) feature excellent temporal coherence and extraordinary high flux at limited transverse coherence. Here, the performance of a SXRL pumped at moderate pump energies is evaluated for CDI and compared to a HHG source. For CDI, a lower bound for the required mutual coherence factor of |μ12| ≥ 0.75 is found by comparing a reconstruction with fixed support to a conventional characterization using double slits. A comparison of the captured diffraction signals suggests that SXRLs have the potential for imaging micron scale objects with sub-20 nm resolution in orders of magnitude shorter integration time compared to a conventional HHG source. Here, the low transverse coherence diameter limits the resolution to approximately 180 nm. The extraordinary high photon flux per laser shot, scalability towards higher repetition rate and capability of seeding with a high harmonic source opens a route for higher performance nanoscale imaging systems based on SXRLs.

A novel technique for divided-pulse amplification is presented in a proof-of-principle experiment. A pulse burst, cut out of the pulse train of a mode-locked oscillator, is amplified and temporally combined into a single pulse. High combination efficiency and excellent pulse contrast are demonstrated. The system is mostly fiber-coupled, enabling a high interferometric stability. This approach provides access to the amplitude and phase of the individual pulses in the burst to be amplified, potentially allowing the compensation of gain saturation and nonlinear phase mismatches within the burst. Therefore, this technique enables the scaling of the peak power and pulse energy of pulsed laser systems beyond currently prevailing limitations.

The energy deposition of ions in dense plasmas is a key process in inertial confinement fusion that determines the α-particle heating expected to trigger a burn wave in the hydrogen pellet and resulting in high thermonuclear gain. However, measurements of ion stopping in plasmas are scarce and mostly restricted to high ion velocities where theory agrees with the data. Here, we report experimental data at low projectile velocities near the Bragg peak, where the stopping force reaches its maximum. This parameter range features the largest theoretical uncertainties and conclusive data are missing until today. The precision of our measurements, combined with a reliable knowledge of the plasma parameters, allows to disprove several standard models for the stopping power for beam velocities typically encountered in inertial fusion. On the other hand, our data support theories that include a detailed treatment of strong ion-electron collisions.

A forwardly-peaked bright neutron source was produced using a laser-driven, deuteron-rich ion beam in a pitcher-catcher scenario. A proton-free ion source was produced via target normal sheath acceleration from Au foils having a thin layer of D₂O ice at the rear side, irradiated by sub-petawatt laser pulses (~200 J, ~750 fs) at peak intensity ∼2×10²⁰ W cm⁻². The neutrons were preferentially produced in a beam of ~70° FWHM cone along the ion beam forward direction, with maximum energy up to ~40 MeV and a peak flux along the axis ∼2×10⁹ n sr⁻¹ for neutron energy above 2.5 MeV. The experimental data is in good agreement with the simulations carried out for the d(d,n)³He reaction using the deuteron beam produced by the ice-layered target.

The discovery of optical solitons being understood as temporally and spectrally stationary optical states has enabled numerous innovations among which, most notably, supercontinuum light sources have become widely used in both fundamental and applied sciences. Here, we report on experimental evidence for dynamics of hybrid solitons—a new type of solitary wave, which emerges as a result of a strong non-instantaneous nonlinear response in CS2-filled liquid-core optical fibres. Octave-spanning supercontinua in the mid-infrared region are observed when pumping the hybrid waveguide with a 460 fs laser (1.95 μm) in the anomalous dispersion regime at nanojoule-level pulse energies. A detailed numerical analysis well correlated with the experiment uncovers clear indicators of emerging hybrid solitons, revealing their impact on the bandwidth, onset energy and noise characteristics of the supercontinua. Our study highlights liquid-core fibres as a promising platform for fundamental optics and applications towards novel coherent and reconfigurable light sources.