Peer-Review Publications

We report on the generation of 17.6 W of visible radiation at 650 nm using four-wave-mixing in an endlessly single-mode silica fiber. The conversion efficiency was as high as ~ 30%. This high efficiency could be obtained by exploiting the natural absorption of silica for the mid-infrared radiation > 2.5µm. In a separate experiment 1.6 W of mid-IR radiation at 2570 nm were generated simultaneously with 14.4 W at 672 nm. These power levels of picosecond red radiation are among the highest reported so far for a diffraction limited beam quality in this wavelength region.

It is shown that the hydrodynamic model of a one-dimensional collisionless plasma expansion is contained in the kinetic description as a special case. This belongs to a specific choice for the electron distribution function. Moreover, the consequences of the use of the hydrodynamic approach regarding the temporal evolution of the electron phase space density are investigated. It turns out that only the case of a hydrodynamic description with the adiabatic constant κ = 3 is physically self-consistent. Numerical simulations confirm this argumentation. The analysis for the case κ = 3 is extended to the kinetics of a relativistic electron gas.

Light beams carrying a point singularity with a screw-type phase distribution are associated with an optical vortex. The corresponding momentum flow leads to an orbital angular momentum of the photons. The study of optical vortices has led to applications such as particle micro-manipulation, imaging, interferometry, quantum information and high-resolution microscopy and lithography. Recent analyses showed that transitions forbidden by selection rules seem to be allowed when using optical vortex beams. To exploit these intriguing new applications, it is often necessary to shorten the wavelength by nonlinear frequency conversion. However, during the conversion the optical vortices tend to break up. Here we show that optical vortices can be generated in the extreme ultraviolet (XUV) region using high-harmonic generation. The singularity impressed on the fundamental beam survives the highly nonlinear process. Vortices in the XUV region have the same phase distribution as the driving field, which is in contradiction to previous findings, where multiplication of the momentum by the harmonic order is expected. This approach opens the way for several applications based on vortex beams in the XUV region.

We present a detailed analysis of the systematic errors that affect single-shot carrier envelope phase (CEP) measurements in experiments with long acquisition times, for which only limited long-term laser stability can be achieved. After introducing a scheme for eliminating these systematic errors to a large extent, we apply our approach to investigate the CEP dependence of the yield of doubly charged ions produced via non-sequential double ionization of argon in strong near-single-cycle laser pulses. The experimental results are compared to predictions of semiclassical calculations.

Fully relativistic treatment of the electron-atom and positron-atom bremsstrahlung is reported. The calculation is based on the partial-wave expansion of the Dirac scattering states in an external atomic field. A comparison of the electron and positron bremsstrahlung is presented for the single and double differential cross sections and the Stokes parameters of the emitted photon. It is demonstrated that the electron-positron symmetry of the bremsstrahlung spectra, which is nearly exact in the nonrelativistic regime, is to a large extent removed by the relativistic effects.

Focal aberrations of large-aperture highly oriented pyrolytic graphite (HOPG) crystals in von-Hàmos geometry are investigated by experimental and computational methods. A mosaic HOPG crystal film of 100 μm thickness diffracts 8 keV x-rays. This thickness is smaller than the absorption depth of the symmetric 004-reflection, which amounts to 257 μm. Cylindrically bent crystals with 110 mm radius of curvature and up to 100 mm collection width produce a X-shaped halo around the focus. This feature vanishes when the collection aperture is reduced, but axial spectral profiles show that the resolution is not affected. X-ray topography reveals significant inhomogeneous crystallite domains of 2 ± 1 mm diameter along the entire crystal. Rocking curves shift by about ±20 arcmin between domains, while their full width at half-maximum varies between 30 and 50 arcmin. These inhomogeneities are not imprinted at the focal spot, since the monochromatically reflecting area of the crystal is large compared to inhomogeneities. Ray-tracing calculations using a Monte-Carlo-based algorithm developed for mosaic crystals reproduce the X-shaped halo in the focal plane, stemming from the mosaic defocussing in the non-dispersive direction in combination with large apertures. The best achievable resolution is found by analyzing a diversity of rocking curve widths, source sizes and crystal thicknesses for 8 keV x-rays to be ΔE/E ~ 10^(−4). Finally a general analytic expression for the shape of the aberration is derived.

Harmonic generation in the limit of ultrasteep density gradients is studied experimentally. Observations reveal that, while the efficient generation of high order harmonics from relativistic surfaces requires steep plasma density scale lengths (L_p/λ < 1), the absolute efficiency of the harmonics declines for the steepest plasma density scale length L_p → 0, thus demonstrating that near-steplike density gradients can be achieved for interactions using high-contrast high-intensity laser pulses. Absolute photon yields are obtained using a calibrated detection system. The efficiency of harmonics reflected from the laser driven plasma surface via the relativistic oscillating mirror was estimated to be in the range of 10^-4 – 10^-6 of the laser pulse energy for photon energies ranging from 20 – 40 eV, with the best results being obtained for an intermediate density scale length.

We show that magnetic fields significantly enhance a new tunneling mechanism in quantum field theories with photons coupling to fermionic minicharged particles (MCPs). We propose a dedicated laboratory experiment of the light-shining-through-walls type that can explore a parameter regime comparable to and even beyond the best model-independent cosmological bounds. With present-day technology, such an experiment is particularly sensitive to MCPs with masses in and below the meV regime as suggested by new-physics extensions of the standard model.

Accurate values of the emission and absorption cross sections of Yb:YAG, Yb:LuAG, and Yb:CaF_2 as a function of temperature between room temperature and 200 °C are presented. For this purpose, absorption and fluorescence spectra were measured using a setup optimized to reduce the effect of radiation trapping. From these data, emission cross sections were retrieved by combining the Fuchtbauer–Ladenburg equation and the reciprocity method. Based on our measurements, simple estimations illustrate the effect of temperature shifts that are likely to occur in typical laser setups. Our results show that even minor temperature variations can have significant impact on the laser performance using Yb:YAG and Yb:LuAG as an active medium, while Yb:CaF_2 appears to be rather insensitive.

In the present work we investigate the sequential radiative recombination (RR) of initially bare ions colliding with two spatially separated electron targets. It is shown that magnetic sublevel population of the hydrogenlike ions, produced by the electron capture from the first target, depends on the emission direction of the (first) RR photon. This population, which can be expressed in terms of the polarization parameters, affects then the angular and polarization properties of the radiation emitted in the collision with the second target. The coincidence measurements of two subsequent RR photons may allow one to understand, therefore, the production and diagnostics of the ion spin polarization. In order to describe this polarization production and diagnostic scheme we derive the general expression for the γ-γ correlation function. Detailed calculations for the dependence of this function on the geometry of photon emission and collision energy are performed for the radiative recombination of bare uranium ions.

We show experimentally that extreme ultraviolet radiation is produced when a laser pulse is Thomson backscattered from sheets of relativistic electrons that are formed at the rear surface of a foil irradiated on its front side with a high-intensity laser. An all-optical setup is realized using the Jena titanium:sapphire ten-terawatt laser system with an enhanced amplified spontaneous emission background of 10^−12. The main pulse is split into two: one of them accelerates electrons from thin aluminium foil targets to energies of the order of some MeV and the other, counterpropagating probe pulse Thomson-backscatters off these electrons when they exit the target rear side. The process produced photons within a wide spectral range of some tens of eV as a result of the broad electron energy distribution. The highest scattering intensity is observed when the probe pulse arrives at the target rear surface 100 fs after irradiation of the target front side by the pump pulse, corresponding to the maximum flux of hot electrons at the interaction region. These results can provide time-resolved information about the evolution of the rear-surface electron sheath and hence about the dynamics of the electric fields responsible for the acceleration of ions from the rear surface of thin, laser-irradiated foils.

We present a Penning trap as a tool for advanced studies of particles in extreme laser fields. Particularly, trap-specific manipulation techniques allow control over the confined particles’ localization and spatial density by use of trap electrodes as ‘electrostatic tweezers’ and by application of a ‘rotating wall’, respectively. It is thereby possible to select and prepare well-defined ion ensembles and to optimize the laser–particle interaction. Non-destructive detection of reaction educts and products with up to single-ion sensitivity supports advanced studies by maintaining the products for further studies at extended confinement times of minutes and above. The trap features endcaps with conical openings for applications with strongly focused lasers. We show that such a modification of a cylindrical trap is possible while harmonicity and tunability are maintained.

We present the setup of a polarization rotating device and its adaption for high-power short-pulse laser systems. Compared to conventional halfwave plates, the all-reflective principle using three zero-phase shift mirrors provides a higher accuracy and a higher damage threshold. Since plan-parallel plates, e.g. these halfwave plates, generate postpulses, which could lead to the generation of prepulses during the subsequent laser chain, the presented device avoids parasitic pulses and is therefore the preferable alternative for high-contrast applications. Moreover the device is easily scalable for large beam diameters and its spectral reflectivity can be adjusted by an appropriate mirror coating to be well suited for ultra-short laser pulses.

Attosecond science is enabled by the ability to convert femtosecond near-infrared laser light into coherent harmonics in the extreme ultraviolet spectral range. While attosecond sources have been utilized in experiments that have not demanded high intensities, substantially higher photon flux would provide a natural link to the next significant experimental breakthrough. Numerical simulations of dual-gas high harmonic generation indicate that the output in the cutoff spectral region can be selectively enhanced without disturbing the single-atom gating mechanism. Here, we summarize the results of these simulations and present first experimental findings to support these predictions.

The electron emission of highly charged ions has been reanalyzed with the goal of separating the magnetic and retardation contributions to the electron-electron (e-e) interaction from the static Coulomb repulsion in strong fields. A remarkable change in the electron angular distribution due to the relativistic terms in the e-e interaction is found, especially for the autoionization of beryllium-like projectiles, following a 1s → 2p_(3/2) Coulomb excitation in collision with some target nuclei. For low-energetic, high-Z projectiles with Tp ≤ 10 MeV u^(−1), a diminished (electron) emission in the forward direction as well as oscillations in the electron angular distribution due to the magnetic and retarded interactions are predicted for the autoionization of the 1s 2s^(2) 2p_(3/2) 3^P_2 resonance into the 1s^2 2s^2 S_(1/2) ground and the 1s^2 2p^2P_(1/2) excited levels of the finally lithium-like ions, and in contrast to a pure Coulomb repulsion between the bound and emitted electrons. The proposed excitation-autoionization process can be observed at existing storage rings and will provide a novel insight into the dynamics of electrons in strong fields.

X-ray spectroscopy is used to obtain single-shot information on electron beam emittance in a low-energy-spread 0.5 GeV-class laser-plasma accelerator. Measurements of betatron radiation from 2 to 20 keV used a CCD and single-photon counting techniques. By matching x-ray spectra to betatron radiation models, the electron bunch radius inside the plasma is estimated to be ~0.1  μm. Combining this with simultaneous electron spectra, normalized transverse emittance is estimated to be as low as 0.1 mm mrad, consistent with three-dimensional particle-in-cell simulations. Correlations of the bunch radius with electron beam parameters are presented.

We report the first experimental observation of terahertz (THz) radiation from the rear surface of a solid target while interacting with an intense laser pulse. Experimental and two-dimensional particle-in-cell simulations show that the observed THz radiation is mostly emitted at large angles to the target normal. Numerical results point out that a large part of the emission originates from a micron-scale plasma sheath at the rear surface of the target, which is also responsible for the ion acceleration. This opens a perspective for the application of THz radiation detection for on-site diagnostics of particle acceleration in laser-produced plasmas.

We have developed an easy-to-use and reliable timing tool to determine the arrival time of an optical laser and a free electron laser (FEL) pulses within the jitter limitation. This timing tool can be used from XUV to X-rays and exploits high FELs intensities. It uses a shadowgraph technique where we optically (at 800 nm) image a plasma created by an intense XUV or X-ray FEL pulse on a transparent sample (glass slide) directly placed at the pump - probe sample position. It is based on the physical principle that the optical properties of the material are drastically changed when its free electron density reaches the critical density. At this point the excited glass sample becomes opaque to the optical laser pulse. The ultra-short and intense XUV or X-ray FEL pulse ensures that a critical electron density can be reached via photoionization and subsequent collisional ionization within the XUV or X-ray FEL pulse duration or even faster. This technique allows to determine the relative arrival time between the optical laser and the FEL pulses in only few single shots with an accuracy mainly limited by the optical laser pulse duration and the jitter between the FEL and the optical laser. Considering the major interest in pump-probe experiments at FEL facilities in general, such a femtosecond resolution timing tool is of utmost importance.

Uniform density and temperature Xe plasmas have been produced over > 4 mm scale-lengths using x-rays generated in a cylindrical Pb cavity. The cavity is 750 μm in depth and diameter, and is heated by a 300 J, 2 ns square, 1054 nm laser pulse focused to a spot size of 200 μm at the cavity entrance. The plasma is characterized by simultaneous imaging Thomson scattering measurements from both the electron and ion scattering features. The electron feature measurement determines the spatial electron density and temperature profile, and using these parameters as constraints in the ion feature analysis allows an accurate determination of the charge state of the Xe ions. The Thomson scattering probe beam is 40 J, 200 ps, and 527 nm, and is focused to a 100 μm spot size at the entrance of the Pb cavity. Each system has a spatial resolution of 25 μm, a temporal resolution of 200 ps (as determined by the probe duration), and a spectral resolution of 2 nm for the electron feature system and 0.025 nm for the ion feature system. The experiment is performed in a Xe filled target chamber at a neutral pressure of 3–10 Torr, and the x-rays produced in the Pb ionize and heat the Xe to a charge state of 20 ± 4 at up to 200 eV electron temperatures.

We study the evolution and interaction of semi-infinite dark beams carrying phase dislocations, where step- and screw-like phase profiles are combined. Similar to dark beams with a finite length, semi-infinite dark beams tend to move in transversal direction with respect to their background beam. In addition, they develop a snake-like instability and optical vortices detach from their bending ends. We are looking for appropriate conditions to control the process of concatenating and crossing the ends of several such semi-infinite dark beams in a way suitable for probe-beam branching and routing in self-defocusing Kerr nonlinear media. Colinear and perpendicular probe beam propagations in the optically-induced guiding structures are modeled and analyzed with respect to the branching efficiency to respective virtual output channels.

Waveform-controlled light fields offer the possibility of manipulating ultrafast electronic processes on sub-cycle timescales. The optical lightwave control of the collective electron motion in nanostructured materials is key to the design of electronic devices operating at up to petahertz frequencies. We have studied the directional control of the electron emission from 95 nm diameter SiO_2 nanoparticles in few-cycle laser fields with a well-defined waveform. Projections of the three-dimensional (3D) electron momentum distributions were obtained via single-shot velocity-map imaging (VMI), where phase tagging allowed retrieving the laser waveform for each laser shot. The application of this technique allowed us to efficiently suppress background contributions in the data and to obtain very accurate information on the amplitude and phase of the waveform-dependent electron emission. The experimental data that are obtained for 4 fs pulses centered at 720 nm at different intensities in the range (1 - 4) × 10^13 W cm^(−2) are compared to quasi-classical mean-field Monte-Carlo simulations. The model calculations identify electron backscattering from the nanoparticle surface in highly dynamical localized fields as the main process responsible for the energetic electron emission from the nanoparticles. The local field sensitivity of the electron emission observed in our studies can serve as a foundation for future research on propagation effects for larger particles and field-induced material changes at higher intensities.

The application of laser accelerated protons or ions for particle therapy has to cope with relatively large energy and angular spreads as well as possibly significant random fluctuations. We suggest a method for combined focusing and energy selection, which is an effective alternative to the commonly considered dispersive energy selection by magnetic dipoles. Our method is based on the chromatic effect of a magnetic solenoid (or any other energy dependent focusing device) in combination with an aperture to select a certain energy width defined by the aperture radius. It is applied to an initial 6D phase space distribution of protons following the simulation output from a Radiation Pressure Acceleration model. Analytical formula for the selection aperture and chromatic emittance are confirmed by simulation results using the TRACEWIN code. The energy selection is supported by properly placed scattering targets to remove the imprint of the chromatic effect on the beam and to enable well-controlled and shot-to-shot reproducible energy and transverse density profiles.

We present a detailed theoretical description of laser driven x-ray parametric amplification, which has been experimentally demonstrated by Seres et al. [Nature Phys. 6 455 (2010)] together with a supporting basic model. The process is based on the parametric interaction of an x-ray photon with a laser accelerated electron in a Coulomb field. With the extended model we are able to estimate the gain cross section also for a finite energy distribution of the interacting electrons as well as to consider dephasing between the electrons and the x-ray field. The improved model is capable of describing the recent experimental findings much more accurately.

The propagation of a relativistic electron with initial energy ≥ 100 MeV in a number of simple one-dimensional laser field configurations with circular polarization is studied by solving the relativistic equation of motion in the Landau–Lifschitz approach to account for the radiation friction force. The radiation back-reaction on the electron dynamics becomes visible at dimensionless field amplitudes a ≥ 10 at these high particle energies. Analytical expressions are derived for the energy and the longitudinal momentum of the electron, the frequency shift of the light scattered by the electron and the particle trajectories. These findings are compared with the numerical solutions of the basic equations. A strong radiation damping effect results in reduced light scattering, forming at the same time a broad quasi-continuous spectrum. In addition, the electron dynamics in the strong field of a quasistationary laser piston is investigated. Analytical solutions for the electron trajectories in this complex field pattern are obtained and compared with the numerical solutions. The radiation friction force may stop a relativistic electron after propagation over several laser wavelengths at high laser field strengths, which supports the formation of a stable piston.

High-order-harmonic-generation yield is remarkably sensitive to driving laser ellipticity, which is interesting from a fundamental point of view as well as for applications. The most well-known example is the generation of isolated attosecond pulses via polarization gating. We develop an intuitive semiclassical model that makes use of the recently measured initial transverse momentum of tunneling ionization. The model is able to predict the dependence of the high-order-harmonic yield on driving laser ellipticity and is in good agreement with experimental results and predictions from a numerically solved time-dependent Schrödinger equation.