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Publications by
Dr. Marco Hornung

All publications of HI Jena

2019

I. Tamer, S. Keppler, J. Körner, M. Hornung, M. Hellwing, F. Schorcht, J. Hein, and M. Kaluza
Modeling of the 3D spatio-temporal thermal profile of joule-class Yb³⁺-based laser amplifiers
High Power Laser Science and Engineering 7, E42 (2019)

Abstract: Thermal profile modification of an active material in a laser amplifier via optical pumping results in a change in the material’s refractive index, and causes thermal expansion and stress, eventually leading to spatial phase aberrations, or even permanent material damage. For this purpose, knowledge of the 3D spatio-temporal thermal profile, which can currently only be retrieved via numerical simulations, is critical for joule-class laser amplifiers to reveal potentially dangerous thermal features within the pumped active materials. In this investigation, a detailed, spatio-temporal numerical simulation was constructed and tested for accuracy against surface thermal measurements of various end-pumped Yb³⁺-doped laser-active materials. The measurements and simulations show an excellent agreement and the model was successfully applied to a joule-class Yb³⁺-based amplifier currently operating in the POLARIS laser system at the Friedrich-Schiller-University and Helmholtz-Institute Jena in Germany.

2018

G. A. Becker, S. Tietze, S. Keppler, J. Reislöhner, J. H. Bin, L. Bock, F.-E. Brack, J. Hein, M. Hellwing, P. Hilz, M. Hornung, A. Kessler, S. D. Kraft, S. Kuschel, H. Liebetrau, W. Ma, J. Polz, H.-P. Schlenvoigt, F. Schorcht, M. B. Schwab, A. Seidel, K. Zeil, U. Schramm, M. Zepf, J. Schreiber, S. Rykovanov, and M. C. Kaluza
Ring-like spatial distribution of laser accelerated protons in the ultra-high-contrast TNSA-regime
Plasma Physics and Controlled Fusion 60, 055010 (2018)

Abstract: The spatial distribution of protons accelerated from submicron-thick plastic foil targets using multi-terawatt, frequency-doubled laser pulses with ultra-high temporal contrast has been investigated experimentally. A very stable, ring-like beam profile of the accelerated protons, oriented around the target’s normal direction has been observed. The ring’s opening angle has been found to decrease with increasing foil thicknesses. Two-dimensional particle-in-cell simulations reproduce our results indicating that the ring is formed during the expansion of the proton density distribution into the vacuum as described by the mechanism of target-normal sheath acceleration. Here—in addition to the longitudinal electric fields responsible for the forward acceleration of the protons—a lateral charge separation leads to transverse field components accelerating the protons in the lateral direction.

I. Tamer, S. Keppler, M. Hornung, J. Körner, J. Hein, and M. C. Kaluza
Spatio-Temporal Characterization of Pump-Induced Wavefront Aberrations in Yb3 + -Doped Materials
Laser & Photonics Reviews 12, 1700211 (2018)

Abstract: Abstract A comprehensive spatio-temporal characterization is presented describing the pump-induced wavefront aberrations in Yb3 + -doped YAG, CaF2, and fluorophosphate glass. Time-resolved interferometric measurements were performed to reveal the profiles of the total optical path differences (OPDs), which are described by the spatio-temporal superposition of thermal as well as electronic contributions, across the free aperture of the considered diode-pumped active materials. These contributions were individually determined by a COMSOL-based thermal profile model along with a detailed characterization of the electronic changes by measuring the single-pass gain and the spatial fluorescence profile. Due to the low quantum defect, the amplitude of the electronic component becomes comparable for all three materials and, in the case of Yb:CaF2, almost completely compensates the thermal component resulting from a pump pulse during the time frame of laser pulse amplification. Finally, all relevant material constants – such as the photoelastic constant and the polarizability difference – could be determined during this investigation, allowing the accurate modeling of the total pump-induced wavefront aberrations and subsequent optimization for laser systems worldwide employing these Yb3 + -doped materials.

2017

H. Liebetrau, M. Hornung, S. Keppler, M. Hellwing, A. Kessler, F. Schorcht, J. Hein, and M. C. Kaluza
Intracavity stretcher for chirped-pulse amplification in high-power laser systems
Optics Letters 42, 326 (2017)

Abstract: We present pulse stretching with an intracavity Offner-type pulse stretcher applied to a high-energy, short-pulse laser system. The compact intracavity design, offering a tunable stretching factor, allows the pulses to be stretched to several nanoseconds and, at the same time, to be amplified to 100 μJ. The stretched pulses have been further amplified with the high-power laser system Polaris and have been recompressed to durations as short as 102 fs, reaching peak powers of 100 TW. Furthermore, the temporal intensity contrast is investigated and compared to the formerly used stretcher setup.

2016

M. Hornung, H. Liebetrau, S. Keppler, A. Kessler, M. Hellwing, F. Schorcht, G. A. Becker, M. Reuter, J. Polz, J. Körner, J. Hein, and M. C. Kaluza
54  J pulses with 18  nm bandwidth from a diode-pumped chirped-pulse amplification laser system
Optics Letters 41, 5413 (2016)

Abstract: We report on results from the fully diode-pumped chirped-pulse amplification laser system Polaris. Pulses were amplified to a maximum energy of 54.2 J before compression. These pulses have a full width at half-maximum spectral bandwidth of 18 nm centered at 1033 nm and are generated at a repetition rate of 0.02 Hz. To the best of our knowledge, these are the most energetic broadband laser pulses generated by a diode-pumped laser system so far. Due to the limited size of our vacuum compressor, only attenuated pulses could be compressed to a duration of 98 fs containing an energy of 16.7 J, which leads to a peak power of 170 TW. These pulses could be focused to a peak intensity of 1.3×1021  W/cm2. Having an ultra-high temporal contrast of 1012 with respect to amplified spontaneous emission these laser pulses are well suited for high-intensity laser–matter experiments.

S. Keppler, M. Hornung, P. Zimmermann, H. Liebetrau, M. Hellwing, J. Hein, and M. C. Kaluza
Tunable filters for precise spectral gain control in ultra-short-pulse laser systems
Optics Letters 41, 4708 (2016)

Abstract: We present tunable spectral filters (TSFs) as a variable and precisely adjustable method to control the spectral gain of short-pulse laser systems. The TSFs provide a small residual spectral phase and a high damage threshold, and generate no pre- or post-pulses. The method is demonstrated for two different laser materials and can be applied as an intracavity compensation in regenerative amplifiers as well as a method for pre-compensation in high-energy multipass amplifiers. With this method, a full width at half-maximum bandwidth of 23.9 nm could be demonstrated in a diode-pumped, 50 J Yb:CaF2 amplifier.

H. Liebetrau, M. Hornung, S. Keppler, M. Hellwing, A. Kessler, F. Schorcht, J. Hein, and M. C. Kaluza
High contrast, 86  fs, 35  mJ pulses from a diode-pumped Yb:glass double-chirped-pulse amplification laser system
Optics Letters 41, 3006 (2016)

Abstract: We demonstrate the generation of 86 fs, 35 mJ, high-contrast laser pulses at 1030 nm with a repetition rate of 1 Hz from a diode-pumped double chirped-pulse amplification setup. The pulses exhibit a spectral bandwidth exceeding 27 nm full width at half-maximum. This could be achieved by using a laser architecture comprising two stages of chirped pulse amplification with a cross-polarized wave generation filter in between, by applying spectral shaping and by increasing the spectral hard-clip of the second stretcher. These are, to the best of our knowledge, the shortest pulses at the mJ level with ultra-high contrast generated with a diode-pumped front end at 1030 nm.

S. Keppler, A. Sävert, J. Körner, M. Hornung, H. Liebetrau, J. Hein, and M. Kaluza
The generation of amplified spontaneous emission in high-power CPA laser systems
Laser & Photonics Reviews 10, 264 (2016)

Abstract: An analytical model is presented describing the temporal intensity contrast determined by amplified spontaneous emission in high-intensity laser systems which are based on the principle of chirped pulse amplification. The model describes both the generation and the amplification of the amplified spontaneous emission for each type of laser amplifier. This model is applied to different solid state laser materials which can support the amplification of pulse durations ≤350 fs . The results are compared to intensity and fluence thresholds, e.g. determined by damage thresholds of a certain target material to be used in high-intensity applications. This allows determining if additional means for contrast improvement, e.g. plasma mirrors, are required for a certain type of laser system and application. Using this model, the requirements for an optimized high-contrast front-end design are derived regarding the necessary contrast improvement and the amplified “clean” output energy for a desired focussed peak intensity. Finally, the model is compared to measurements at three different high-intensity laser systems based on Ti:Sapphire and Yb:glass. These measurements show an excellent agreement with the model.

2015

M. Hornung, G. Becker, A. Seidel, J. Reislöhner, H. Liebetrau, L. Bock, S. Keppler, A. Kessler, M. Zepf, J. Hein, and M. Kaluza
Generation of 25-TW Femtosecond Laser Pulses at 515 nm with Extremely High Temporal Contrast
Applied Sciences 5, 1970 (2015)

Abstract: We report on the frequency doubling of femtosecond laser pulses at 1030 nm center wavelength generated from the fully diode-pumped laser system POLARIS. The newly generated pulses at a center wavelength of 515 nm have a pulse energy of 3 J with a pulse duration of 120 fs. On the basis of initially ultra-high contrast seed pulses we expect a temporal intensity contrast better 10^17 200 ps before the peak of the main pulse. We analyzed the temporal intensity contrast from milliseconds to femtoseconds with a dynamic range covering more than 20 orders of magnitude. The pulses were focussed with a f/2-focussing parabola resulting in a peak intensity exceeding 10^20 W/cm2. The peak power and intensity are to the best of our knowledge the highest values for 515 nm-laser-pulses achieved so far.

2014

H. Liebetrau, M. Hornung, A. Seidel, M. Hellwing, A. Kessler, S. Keppler, F. Schorcht, J. Hein, and M. C. Kaluza
Ultra-high contrast frontend for high peak power fs-lasers at 1030 nm
Optics Express 22, 24776 (2014)

Abstract: We present the results from a new frontend within a double-chirped pulse amplification architecture (DCPA) utilizing crossed-polarized wave generation (XPW) for generating ultra-high contrast, 150 μJ-level, femtosecond seed pulses at 1030 nm. These pulses are used in the high energy class diode-pumped laser system Polaris at the Helmholtz Institute in Jena. Within this frontend, laser pulses from a 75 MHz oscillator-pulse train are extracted at a repetition rate of 1 Hz, temporally stretched, amplified and then recompressed reaching a pulse energy of 2 mJ, a bandwidth of 12 nm and 112 fs pulse duration at a center wavelength of 1030 nm. These pulses are temporally filtered via XPW in a holographic-cut BaF2 crystal, resulting in 150 μJ pulse energy with an efficiency of 13 %. Due to this non-linear filtering, the relative intensity of the amplified spontaneous emission preceding the main pulse is suppressed to 2×10^−13. This is, to the best of our knowledge, the lowest value achieved in a high peak power laser system operating at 1030 nm center wavelength.

R. Bödefeld, M. Hornung, J. Hein, and M. C. Kaluza
High precision elimination of angular chirp in CPA laser systems with large stretching factors or high bandwidth
Applied Physics B 115, 419 (2014)

Abstract: We present a novel and highly sensitive method to determine the residual angular dispersion of high-power laser pulses after stretching, amplification, and re-compression of the pulses in a chirped-pulse amplification laser system. This method is based on the intentional deflection of a part of the the spectrum within the compressor and aligning the centers of gravity of the two resulting and separated foci with largest possible spectral separation in the far field. Using this technique, we were able to reduce the residual angular dispersion on pulses to less than 0.05 μrad/nm in the vertical plane and less than 0.03 μrad/nm in the horizontal plane, respectively. With this method, it is possible to minimize the deviation of the actual peak intensity for the focused laser pulses to less than 2% of its theoretical limit.

M. Hornung, H. Liebetrau, A. Seidel, S. Keppler, A. Kessler, J. Körner, M. Hellwing, F. Schorcht, D. Klöpfel, A. K. Arunachalam, G. A. Becker, A. Sävert, J. Polz, J. Hein, and M. C. Kaluza
The all-diode-pumped laser system POLARIS – an experimentalist’s tool generating ultra-high contrast pulses with high energy
High Power Laser Science and Engineering 2, e20 (2014)

Abstract: The development, the underlying technology and the current status of the fully diode-pumped solid-state laser system POLARIS is reviewed. Currently, the POLARIS system delivers 4 J energy, 144 fs long laser pulses with an ultra-high temporal contrast of 5×10^12 for the ASE, which is achieved using a so-called double chirped-pulse amplification scheme and cross-polarized wave generation pulse cleaning. By tightly focusing, the peak intensity exceeds 3.5×10^20 W cm^{−2}. These parameters predestine POLARIS as a scientific tool well suited for sophisticated experiments, as exemplified by presenting measurements of accelerated proton energies. Recently, an additional amplifier has been added to the laser chain. In the ramp-up phase, pulses from this amplifier are not yet compressed and have not yet reached the anticipated energy. Nevertheless, an output energy of 16.6 J has been achieved so far.

C. Wandt, S. Klingebiel, S. Keppler, M. Hornung, M. Loeser, M. Siebold, C. Skrobol, A. Kessel, S. Trushin, Z. Major, J. Hein, M. C. Kaluza, F. Krausz, and S. Karsch
Development of a Joule-class Yb:YAG amplifier and its implementation in a CPA system generating 1 TW pulses
Laser & Photonics Reviews 8, 875 (2014)

Abstract: In this paper the development and implementation of a novel amplifier setup as an additional stage for the CPA pump laser of the Petawatt Field Synthesizer, currently developed at the Max-Planck-Institute of Quantum Optics, is presented. This amplifier design comprises 20 relay-imaged passes through the active medium which are arranged in rotational symmetry. As the gain material, an in-house-developed Yb:YAG active-mirror is used. With this setup, stretched 4 ns seed pulses are amplified to output energies exceeding 1 J with repetition rates of up to 2 Hz. Furthermore, a spectral bandwidth of 3.5 nm (FWHM) is maintained during amplification and the compression of the pulses down to their Fourier-limit of 740 fs is achieved. To the best of our knowledge, this is the first demonstration of 1 TW pulses generated via CPA in diode-pumped Yb:YAG.

S. Keppler, M. Hornung, R. Bödefeld, A. Sävert, H. Liebetrau, J. Hein, and M. C. Kaluza
Full characterization of the amplified spontaneous emission from a diode-pumped high-power laser system
Optics Express 22, 11228 (2014)

Abstract: We present the first complete temporal and spatial characterization of the amplified spontaneous emission (ASE) of laser radiation generated by a diode-pumped high-power laser system. The ASE of the different amplifiers was measured independently from the main pulse and was characterized within a time window of \minus10ms \leq t \leq 10ms and an accuracy of up to 15fs around the main pulse. Furthermore, the focusability and the energy of the ASE from each amplifier was measured after recompression. Using our analysis method, the laser components, which need to be optimized for a further improvement of the laser contrast, can be identified. This will be essential for laser-matter interaction experiments requiring a minimized ASE intensity or fluence.

A. Kessler, M. Hornung, S. Keppler, F. Schorcht, M. Hellwing, H. Liebetrau, J. Körner, A. Sävert, M. Siebold, M. Schnepp, J. Hein, and M. C. Kaluza
16.6 J chirped femtosecond laser pulses from a diode-pumped Yb:CaF2 amplifier
Optics Letters 39, 1333 (2014)

Abstract: We report the amplification of laser pulses at a center wavelength of 1034 nm to an energy of 16.6 J from a fully diode-pumped amplifier using Yb:CaF2 as the active medium. Pumped by a total optical power of 300 kW from high-power laser diodes, a gain factor of g=6.1 was achieved in a nine-pass amplifier configuration agreeing with numerical simulations. A measured spectral bandwidth of 10 nm full width at half-maximum promises a bandwidth-limited compression of the pulses down to a duration of 150 fs. These are, to our knowledge, the most energetic laser pulses achieved from a diode-pumped chirped-pulse amplifier so far.

2013

S. Keppler, C. Wandt, M. Hornung, R. Bödefeld, A. Kessler, A. Sävert, M. Hellwing, F. Schorcht, J. Hein, and M. C. Kaluza
Multipass amplifiers of POLARIS
Proceedings of SPIE 8780, 87800I (2013)

Abstract: Advanced high intensity laser matter interaction experiments always call for optimized laser performance. In order to further enhance the POLARIS laser system, operational at the University of Jena and the Helmholtz-Institute Jena, in particular its energy, bandwidth and focusability, new amplifier technologies have been developed and are reported here. Additionally, existing sections were considerably improved. A new multi-pass amplification stage, which is able to replace two currently used ones, was developed in close collaboration with the MPQ (Garching). The new basic elements of this amplifier are well homogenized pump modules and the application of a successive imaging principle. By operating the amplifier under vacuum conditions a top hat beam profile with an output energy of up to 1.5 J per pulse is foreseen. The already implemented POLARIS amplifier A4 was further improved by adapting an advanced method for the homogenization of the multi-spot composed pump profile. The new method comprises a computer-based evolutionary algorithm which optimizes the position of the different spots regarding its individual size, shape and intensity. The latter allowed a better homogenization of the POLARIS near field profile.

M. Hornung, S. Keppler, R. Bödefeld, A. Kessler, H. Liebetrau, J. Körner, M. Hellwing, F. Schorcht, O. Jäckel, A. Sävert, J. Polz, A. K. Arunachalam, J. Hein, and M. C. Kaluza
High-intensity, high-contrast laser pulses generated from the fully diode-pumped Yb:glass laser system POLARIS
Optics Letters 38, 718 (2013)

Abstract: We report on the first generation of high-contrast, 164 fs duration pulses from the laser system POLARIS reaching focused peak intensities in excess of 2×10^20  W/cm2. To our knowledge, this is the highest peak intensity reported so far that has been achieved with a diode-pumped, solid-state laser. Several passive contrast enhancement techniques have been specially developed and implemented, achieving a relative prepulse intensity smaller than 10^−8 at t=−30  ps before the main pulse. Furthermore a closed-loop adaptive-optics system has been installed. Together with angular chirp compensation, this method has led to a significant reduction of the focal spot size and an increase of the peak intensity.

2012

S. Keppler, M. Hornung, R. Bödefeld, M. Kahle, J. Hein, and M. C. Kaluza
All-reflective, highly accurate polarization rotator for high-power short-pulse laser systems
Optics Express 20, 20742 (2012)

Abstract: We present the setup of a polarization rotating device and its adaption for high-power short-pulse laser systems. Compared to conventional halfwave plates, the all-reflective principle using three zero-phase shift mirrors provides a higher accuracy and a higher damage threshold. Since plan-parallel plates, e.g. these halfwave plates, generate postpulses, which could lead to the generation of prepulses during the subsequent laser chain, the presented device avoids parasitic pulses and is therefore the preferable alternative for high-contrast applications. Moreover the device is easily scalable for large beam diameters and its spectral reflectivity can be adjusted by an appropriate mirror coating to be well suited for ultra-short laser pulses.

2011

S. Keppler, R. Bödefeld, M. Hornung, A. Sävert, J. Hein, and M. C. Kaluza
Prepulse suppression in a multi-10-TW diode-pumped Yb:glass laser
Applied Physics B 104, 11 (2011)

Abstract: We describe a novel method to improve the temporal intensity contrast (TIC) between the main pulse and prepulses in a high-power chirped-pulse amplification (CPA) laser system. Pre- and post-pulses originating from the limited extinction ratio of the polarization gating equipment are suppressed by carefully adjusting the round-trip times of the regenerative amplifiers (RAs) with respect to the oscillator. As a result, leaking pulses from earlier or later round-trips in the RAs are hidden below the temporal shape of the main pulse. The synchronization can easily be controlled by a contrast measurement on a picosecond time scale using a third-order cross-correlator that enables a sub-mm precise adjustment of the cavity lengths. Finally, a method based on spectral interference is introduced that can be used for a fine-adjustment of the cavity lengths for the daily operation, making this new method easy to implement into existing laser systems.

S. Keppler, R. Bödefeld, M. Hornung, A. Sävert, J. Hein, and M. C. Kaluza
Contrast improvement by prepulse suppression in cascaded amplifier cavities
Proc. SPIE (2011)

Abstract: We introduce a method to suppress prepulses of pulse picking systems due to the limited extinction ratio of polarization gating systems. By matching the round trip times of the oscillator and the subsequent regenerative amplifiers, leaking pulses are hidden below the temporal intensity pedestal of the main pulse. With this method, prepulses at the temporal position equal to the time difference of the round trip times of the cavities could be suppressed completely.

2010

M. Hornung, R. Bödefeld, M. Siebold, A. Kessler, M. Schnepp, R. Wachs, A. Sävert, S. Podleska, S. Keppler, J. Hein, and M. C. Kaluza
Temporal pulse control of a multi-10 TW diode-pumped Yb:Glass laser
Applied Physics B 101, 93 (2010)

Abstract: At the Institute of Optics and Quantum Electronics in Jena, Germany, the currently most powerful diode-pumped solid-state laser system with 25-TW peak power Polaris is in operation. In this paper we give an overview about the dispersion management of the chirped pulse amplification in order to minimize the pulse duration and thus to maximize the intensity available for experiments. A detailed description of the stretcher and compressor design with a novel alignment routine is given as well as measurements for the pulse duration and the temporal contrast. The far field measurement of the beam focussed by an off-axis parabola yields a nearly diffraction limited focal spot.

M. Hornung, R. Bödefeld, A. Kessler, J. Hein, and M. C. Kaluza
Spectrally resolved and phase-sensitive far-field measurement for the coherent addition of laser pulses in a tiled grating compressor
Optics Letters 35, 2073 (2010)

Abstract: We describe a method that can be used for the coherent addition of laser pulses. As different laser pulses are initially generated in a laser-pulse compressor equipped with a tiled grating, such a coherent addition is indispens able in order to maximize the intensity in the laser far field. We present measurements in this context where, up to now, an unavoidable difference in the grating constants between the phased gratings reduced the maximum achievable intensity. The method significantly facilitates the high-precision alignment of a tiled grating compressor and could also be used for a coherent addition of laser pulses.

J. Hein, M. Hornung, R. Bödefeld, S. Podleska, A. Sävert, R. Wachs, A. Kessler, S. Keppler, M. Wolf, J. Polz, O. Jäckel, M. Nicolai, M. Schnepp, J. Körner, M. C. Kaluza, and G. G. Paulus
Multiterawatt peak power generated by the all diode pumped laser—POLARIS
AIP Conference Proceedings 1228, 159 (2010)

Abstract: At the Institute of Optics and Quantum Electronics, University of Jena, a fully diode pumped ultrahigh peak power laser system—POLARIS—has been realized. Presently, this laser system reaches a peak power of some ten terawatt. The last amplifier, which will boost the output energy to the 100 J level, is nearly completed and will be soon commissioned. The applied technologies and the basic design are reviewed here.