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Referierte Publikationen


2022

F. Karbstein
Large N external-field quantum electrodynamics
Journal of High Energy Physics 01, 057 (2022)

Abstract: We advocate the study of external-field quantum electrodynamics with N charged particle flavors. Our main focus is on the Heisenberg-Euler effective action for this theory in the large N limit which receives contributions from all loop orders. The contributions beyond one loop stem from one-particle reducible diagrams. We show that specifically in constant electromagnetic fields the latter are generated by the one-loop Heisenberg-Euler effective Lagrangian. Hence, in this case the large N Heisenberg-Euler effective action can be determined explicitly at any desired loop order. We demonstrate that further analytical insights are possible for electric-and magnetic-like field configurations characterized by the vanishing of one of the secular invariants of the electromagnetic field and work out the all-orders strong field limit of the theory.

2021

S. Skruszewicz, A. Przystawik, D. Schwickert, M. Sumfleth, M. Namboodiri, V. Hilbert, R. Klas, P. Gierschke, V. Schuster, A. Vorobiov, C. Haunhorst, D. Kip, J. Limpert, J. Rothhardt, and T. Laarmann
Table-top interferometry on extreme time and wavelength scales
Optics Express 29, 40333 (2021)

Abstract: High-resolution Fourier-transform spectroscopy using table-top sources in the extreme ultraviolet (XUV) spectral range is still in its infancy. In this contribution a significant advance is presented based on a Michelson-type all-reflective split-and-delay autocorrelator operating in a quasi amplitude splitting mode. The autocorrelator works under a grazing incidence angle in a broad spectral range (10 nm - 1 µ m) providing collinear propagation of both pulse replicas and thus a constant phase difference across the beam profile. The compact instrument allows for XUV pulse autocorrelation measurements in the time domain with a single-digit attosecond precision resulting in a resolution of E/Δ E=2000. Its performance for spectroscopic applications is demonstrated by characterizing a very sharp electronic transition at 26.6 eV in Ar gas induced by the 11th harmonic of a frequency-doubled Yb-fiber laser leading to the characteristic 3s3p⁶4p¹P¹ Fano-resonance of Ar atoms. We benchmark our time-domain interferometry results with a high-resolution XUV grating spectrometer and find an excellent agreement. The common-path interferometer opens up new opportunities for short-wavelength femtosecond and attosecond pulse metrology and dynamic studies on extreme time scales in various research fields.

L. Du, F. Roeder, Y. Li, M. Shalaby, B. Beleites, F. Ronneberger, and A. Gopal
Organic crystal-based THz source for complex refractive index measurements of window materials using single-shot THz spectroscopy
Applied Physics A 127, 846 (2021)

Abstract: We employed N-benzyl-2-methyl-4-nitroaniline (BNA) crystals bonded on substrates of different thermal conductivity to generate THz radiation by pumping with 800 nm laser pulses. Crystals bonded on sapphire substrate provided four times more THz yield than glass substrate. A pyrodetector and a single-shot electro-optic (EO) diagnostic were employed for measuring the energy and temporal characterisation of the THz pulse. Systematic studies were carried out for the selection of a suitable EO crystal, which allowed accurate determination of the emitted THz spectrum from both substrates. Subsequently, the THz source and single-shot electro-optic detection scheme were employed to measure the complex refractive index of window materials in the THz range.

G. Gaigalas, and S. Fritzsche
Angular coefficients for symmetry-adapted configuration states in jj-coupling
Computer Physics Communications 267, 108086 (2021)

Abstract: In atomic structure and collision theory, the efficient spin-angular integration is known to be crucial and often decides, how accurate the properties and behavior of atoms can be predicted numerically. Various methods have been developed in the past to keep the computation (and implementation) of the spin-angular integration feasible for complex shell structures, including open d- and f-shell elements. To support such computations, we here provide a new implementation of the angular coefficients for jjcoupled and symmetry-adapted configuration states that is entirely built upon the quasi-spin formalism. The moduleSpinAngularis based on Julia, a new programming language for scientific computing, and supports a simple access to all (completely) reduced tensors, coefficients of fractional parentage for subshells with j <= 9/2 as well as the re-coupling coefficients from this formalism. Moreover, this module has been worked out for multiple purposes, including 1) the accurate calculation of atomic properties, 2) further studies on spin-angular integration theory, 3) the development of new or existing computer programs as well as 4) the manipulation of reduced matrix elements from this theory. The present implementation will therefore help advance the algebraic evaluation of many-electron (transition) amplitudes and to apply the theory to newly emerging research areas.

F. C. Salgado, K. Grafenstein, A. Golub, A. Dopp, A. Eckey, D. Hollatz, C. Muller, A. Seidel, D. Seipt, S. Karsch, and M. Zepf
Towards pair production in the non-perturbative regime
New Journal of Physics 23, 105002 (2021)

Abstract: The interaction of light with the quantum-vacuum is predicted to give rise to some of the most fundamental and exotic processes in modern physics, which remain untested in the laboratory to date. Electron-positron pair production from a pure vacuum target, which has yet to be observed experimentally, is possibly the most iconic. The advent of ultra-intense lasers and laser accelerated GeV electron beams provide an ideal platform for the experimental realisation. Collisions of high energy gamma-ray photons derived from the GeV electrons and intense laser fields result in detectable pair production rates at field strengths that approach and exceed the Schwinger limit in the centre-of-momentum frame. A detailed experiment has been designed to be implemented at the ATLAS laser at the centre of advanced laser applications. We show full calculations of the expected backgrounds and beam parameters which suggest that single pair events can be reliably generated and detected.

J. Buldt, H. Stark, M. Mueller, C. Grebing, C. Jauregui, and J. Limpert
Gas-plasma-based generation of broadband terahertz radiation with 640 mW average power
Optics Letters 46, 5256 (2021)

Abstract: We present a high-power source of broadband terahertz (THz) radiation covering the whole THz spectral region (0.1-30 THz). The two-color gas plasma generation process is driven by a state-of-the-art ytterbium fiber chirped pulse amplification system based on coherent combination of 16 rod-type amplifiers. Prior to the THz generation, the pulses are spectrally broadened in a multipass cell and compressed to 37 fs with a pulse energy of 1.3 mJ at a repetition rate of 500 kHz. A gas-jet scheme has been employed for the THz generation, increasing the efficiency of the process to 0.1%. The air-biased coherent detection scheme is implemented to characterize the full bandwidth of the generated radiation. A THz average power of 640 mW is generated, which is the highest THz average power achieved to date. This makes this source suitable for a variety of applications, e.g., spectroscopy of strongly absorbing samples or driving nonlinear effects for the studies of material properties.

D. Wanisch, and S. Fritzsche
Delocalization of quantum information in long-range interacting systems
Physical Review A 104, 042409 (2021)

Abstract: We investigate the delocalization of quantum information in the nonequilibrium dynamics of the XY spin chain with asymptotically decaying interactions similar to 1/r(alpha). As a figure of merit, we employ the tripartite mutual information (TMI), the sign of which indicates if quantum information is predominantly shared globally. Interestingly, the sign of the TMI distinguishes regimes of the exponent a that are known for different behaviors of information propagation. While an effective causal region bounds the propagation of information, if interactions decay sufficiently fast, this information is mainly delocalized, which leads to the necessity of global measurements. Furthermore, the results indicate that mutual information is monogamous for all possible partitionings in this case, implying that quantum entanglement is the dominant correlation. If interactions decay sufficiently slow, though information can propagate (quasi-)instantaneously, it is mainly accessible by local measurements at early times. Furthermore, it takes some finite time until correlations start to become monogamous, which suggests that entanglement is not the dominant correlation at early times. Our findings give new insights into the dynamics and structure of quantum information in many-body systems with long-range interactions, and might get verified on state-of-the-art experimental platforms.

F. Karbstein, and R. Oude Weernink
X-ray vacuum diffraction at finite spatiotemporal offset
Physical Review D 104, 076015 (2021)

Abstract: We study the nonlinear QED signature of x-ray vacuum diffraction in the head-on collision of optical high-intensity and x-ray free-electron laser pulses at finite spatiotemporal offsets between the laser foci. The high-intensity laser driven scattering of signal photons outside the forward cone of the x-ray probe constitutes a prospective experimental signature of quantum vacuum nonlinearity. Resorting to a simplified phenomenological ad hoc model, it was recently argued that the angular distribution of the signal in the far-field is sensitive to the wavefront curvature of the probe beam in the interaction region with the high-intensity pump. In this work, we model both the pump and probe fields as pulsed paraxial Gaussian beams and reanalyze this effect from first principles. We focus on vacuum diffraction both as an individual signature of quantum vacuum nonlinearity and as a potential means to improve the signal-to-background separation in vacuum birefringence experiments.

M. Chambonneau, M. Blothe, Q. Li, V. Fedorov, T. Heuermann, M. Gebhardt, C. Gaida, S. Tertelmann, F. Sotier, J. Limpert, S. Tzortzakis, and S. Nolte
Transverse ultrafast laser inscription in bulk silicon
Physical Review Research 3, 043037 (2021)

Abstract: In-volume ultrafast laser direct writing of silicon is generally limited by strong nonlinear propagation effects preventing the production of modifications. By using advantageous spectral, temporal, and spatial conditions, we demonstrate that modifications can be repeatably produced inside silicon. Our approach relies on irradiation at approximate to 2 mu m wavelength with temporally distorted femtosecond pulses. These pulses are focused in a way that spherical aberrations of different origins mutually balance, as predicted by point spread function analyses and in good agreement with nonlinear propagation simulations. We also establish the laws governing modification growth on a pulse-to-pulse basis, which allows us to demonstrate transverse inscription inside silicon with various line morphologies depending on the irradiation conditions. We finally show that the production of single-pulse repeatable modifications is a necessary condition for reliable transverse inscription inside silicon.

M. Almassarani, S. Meng, B. Beleites, F. Ronneberger, G. Paulus, and A. Gopal
Parametric Study of Proton Acceleration from Laser-Thin Foil Interaction
Plasma 4, 670 (2021)

Abstract: We experimentally investigated the accelerated proton beam characteristics such as maximum energy and number by varying the incident laser parameters. For this purpose, we varied the laser energy, focal spot size, polarization, and pulse duration. The proton spectra were recorded using a single-shot Thomson parabola spectrometer equipped with a microchannel plate and a high-resolution charge-coupled device with a wide detection range from a few tens of keV to several MeV. The outcome of the experimental findings is discussed in detail and compared to other theoretical works.

F. Karbstein
Derivative corrections to the Heisenberg-Euler effective action
Journal of High Energy Physics 09, 070 (2021)

Abstract: We show that the leading derivative corrections to the Heisenberg-Euler effective action can be determined efficiently from the vacuum polarization tensor evaluated in a homogeneous constant background field. After deriving the explicit parameter-integral representation for the leading derivative corrections in generic electromagnetic fields at one loop, we specialize to the cases of magnetic- and electric-like field configurations characterized by the vanishing of one of the secular invariants of the electromagnetic field. In these cases, closed-form results and the associated all-orders weak-and strong-field expansions can be worked out. One immediate application is the leading derivative correction to the renowned Schwinger-formula describing the decay of the quantum vacuum via electron-positron pair production in slowly-varying electric fields.

B. Ying, F. Machalett, V. Huth, M. Kuebel, A. Sayler, T. Stoehlker, G. Paulus, and P. Wustelt
Experimental study of the laser-induced ionization of heavy metal and metalloid ions: Au+ and Si2+ in intense and sculpted femtosecond laser fields
Journal of Physics B: Atomic, Molecular and Optical Physics 54, 174002 (2021)

Abstract: We implement a liquid metal ion source in a 3D coincidence momentum spectroscopy setup for studying the interaction of ionic targets with intense laser pulses. Laser intensities of up to 4 . 10(16) W cm(-2) allow for the observation of up to ten-fold ionization of Au+-ions and double ionization of Si2+-ions. Further, by utilizing two-color sculpted laser fields to control the ionization process on the attosecond time scale, we demonstrate the capability to resolve the recoil ion momenta of heavy metal atoms. Simulations based on a semiclassical model assuming purely sequential ionization reproduce the experimental data well. This work opens up the use of a range of metallic and metalloid ions, which have hardly been investigated in strong-field laser physics so far.

A.-L. Viotti, S. Alisauskas, H. Tuennermann, E. Escoto, M. Seidel, K. Dudde, B. Manschwetus, I. Hartl, and C. Heyl
Temporal pulse quality of a Yb:YAG burst-mode laser post-compressed in a multi-pass cell
Optics Letters 46, 4686 (2021)

Abstract: Nonlinear pulse post-compression represents an efficient method for ultrashort, high-quality laser pulse production. The temporal pulse quality is, however, limited by amplitude and phase modulations intrinsic to post-compression. We here characterize in frequency and time domain with high dynamic range individual post-compressed pulses within laser bursts comprising 100-kHz-rate pulse trains. We spectrally broaden 730 fs, 3.2 mJ pulses from a Yb:YAG laser in a gas-filled multi-pass cell and post-compress them to 56 fs. The pulses exhibit a nearly constant energy content of 78% in the main peak over the burst plateau, which is close to the theoretical limit. Our results demonstrate attractive pulse characteristics, making multi-pass post-compressed lasers very applicable for pump-probe spectroscopy at, e.g., free-electron lasers or as efficient drivers for secondary frequency conversion stages.

A. Mueller, M. Martins, J. Borovik, T. Buhr, A. Perry-Sassmannshausen, S. Reinwardt, F. Trinter, S. Schippers, S. Fritzsche, and A. S. Kheifets
Role of L-shell single and double core-hole production and decay in m-fold (1 <= m <= 6) photoionization of the Ar+ ion
Physical Review A 104, 033105 (2021)

Abstract: Multiple ionization of the Ar+(3s(2)3p(5)) ion by a single photon has been investigated in the photon-energy range 250-1800 eV employing the photon-ion merged-beams technique. Absolute partial cross sections were measured for all Ar(1+m)+ product-ion channels with 1 <= m <= 6 covering a size range from several tens of Mb down to a few b. Narrow 2p-subshell excitation resonances were observed in all channels up to quadruple ionization at a photon-energy bandwidth of 52 meV. Double excitations involving a 2p and a 3s or 3p electron were also studied at high resolution and the measurements of the broad 2s excitation resonances directly showed their natural widths. Contributions of direct photo double ionization (PDI) to the production of the highest final Ar ion charge states are revealed, with PDI of the 2s subshell being mainly responsible for the production of Ar7+. The experiment made use of the PIPE setup installed at beamline P04 of the PETRA III synchrotron light source of DESY in Hamburg. The measurements were supported by theoretical calculations to identify the main contributions to the observed cross sections. Comparisons of theory and experiment show remarkable agreement but also hint to additional ionizationmechanisms that are not considered in the theoretical models such as core ionization accompanied by excitations with subsequent Auger decays leading to net m-fold ionization with m >= 4.

S. Fritzsche
Symbolic Evaluation of Expressions from Racah s Algebra
Symmetry 13, 1558 (2021)

Abstract: Based on the rotational symmetry of isolated quantum systems, Racah s algebra plays a significant role in nuclear, atomic and molecular physics, and at several places elsewhere. For N-particle (quantum) systems, for example, this algebra helps carry out the integration over the angular coordinates analytically and, thus, to reduce them to systems with only N (radial) coordinates. However, the use of Racah s algebra quickly leads to complex expressions, which are written in terms of generalized Clebsch-Gordan coefficients, Wigner n-j symbols, (tensor) spherical harmonics and/or rotation matrices. While the evaluation of these expressions is straightforward in principle, it often becomes laborious and prone to making errors in practice. We here expand Jac, the Jena Atomic Calculator, to facilitate the sum-rule evaluation of typical expressions from Racah s algebra. A set of new and revised functions supports the simplification and subsequent use of such expressions in daily research work or as part of lengthy derivations. A few examples below show the recoupling of angular momenta and demonstrate how Jac can be readily applied to find compact expressions for further numerical studies. The present extension makes Jac a more flexible and powerful toolbox in order to deal with atomic and quantum many-particle systems.

F. Karbstein, C. Sundqvist, K. S. Schulze, I. Uschmann, H. Gies, and G. G. Paulus
Vacuum birefringence at x-ray free-electron lasers
New Journal of Physics 23, 095001 (2021)

Abstract: We study the perspectives of measuring the phenomenon of vacuum birefringence predicted by quantum electrodynamics using an x-ray free-electron laser (XFEL) alone. We devise an experimental scheme allowing two consecutive XFEL pulses to collide under a finite angle, and thus act as both pump and probe field for the effect. The signature of vacuum birefringence is encoded in polarization-flipped signal photons to be detected with high-purity x-ray polarimetry. Our findings for idealized scenarios underline that the discovery potential of solely XFEL-based setups can be comparable to those involving optical high-intensity lasers. For currently achievable scenarios, we identify several key details of the x-ray optical ingredients that exert a strong influence on the magnitude of the desired signatures.

M. Mueller, C. Aleshire, J. Buldt, H. Stark, C. Grebing, A. Klenke, and J. Limpert
Scaling potential of beam-splitter-based coherent beam combination
Optics Express 29, 27900 (2021)

Abstract: The impact of nonlinear refraction and residual absorption on the achievable peakand average power in beam-splitter-based coherent beam combination is analyzed theoretically. While the peak power remains limited only by the aperture size, a fundamental average power limit is given by the thermo-optical and thermo-mechanical properties of the beam splitter material and its coatings. Based on our analysis, 100 kW average power can be obtained with state-of-the-art optics at maintained high beam quality (M-2 <= 1.1) and at only 2% loss of combining efficiency. This result indicates that the power-scaling potential of today\textquotesingle s beam-splitter-based coherent beam combination is far from being depleted. A potential scaling route to megawatt-level average power is discussed for optimized beam splitter geometry.

B. Lei, D. Seipt, M. Shi, B. Liu, J. Wang, M. Zepf, and S. Rykovanov
Relativistic modified Bessel-Gaussian beam generated from plasma-based beam braiding
Physical Review A 104, 021501 (2021)

Abstract: We theoretically and numerically demonstrate the generation of a relativistic modified Bessel-Gaussian beam (MBGB) via plasma-based beam braiding. It is realized by injecting several intense Gaussian pulses with well-designed offsets and angles into an underdense plasma channel which acts as a laser-pulse combiner via refractive coupling. The MBGB propagates stably in the plasma channel with a well-controlled orbital angular momentum of large value, exciting a twisted plasma wave. After leaving the plasma, it becomes unguided and survives in vacuum for at least hundreds of femtoseconds. This method is insensitive to the initial laser injection conditions and thus should be robust for experimental implementation. It provides an alternative approach in generating high-quality tunable intense optical vortex beams which are desired for various applications.

Y. Zhang, C. L. Zhong, S. P. Zhu, X. T. He, M. Zepf, and B. Qiao
Obtaining Intense Attosecond Pulses in the Far Field from Relativistic Laser-Plasma Interactions
Physical Review Applied 16, 024042 (2021)

Abstract: In this paper, we show that the Gouy phase shift plays a key role in the far-field waveform evolution of the reflected harmonic radiations from plasma surfaces driven by a relativistic Gaussian laser. With a proper adjustment of laser focal position away from the plasma surface, the inherent separations between the peaks of different harmonic carrier waves as well as the fundamental wave due to different wavelengths can be cleared away when they propagate from near to far field, since they experience the same Gouy phase shift of pi/2. Using this method, intense attosecond pulses can be obtained in the far field with no need of any spectral filters. Three-dimensional particle-in-cell simulations show that far-field attosecond pulses with intensity of 4 x 1015 W/cm2 (2.56 x 1017 W/sr; 65 times increase) and duration of 76 as (50% decrease) can be obtained by lasers at intensities of 1021 W/cm2. Such brilliant pulses with fully reserved spectra significantly benefit applications in attosecond science.

A. Koszorus, L. J. Vormawah, R. Beerwerth, M. L. Bissell, P. Campbell, B. Cheal, C. S. Devlin, T. Eronen, S. Fritzsche, S. Geldhof, H. Heylen, J. D. Holt, A. Jokinen, S. Kelly, I. D. Moore, T. Miyagi, S. Rinta-Antila, A. Voss, and C. Wraith
Proton-neutron pairing correlations in the self-conjugate nucleus Sc-42
Physical Review B 819, 136439 (2021)

Abstract: Collinear laser spectroscopy of the N = Z = 21 self-conjugate nucleus Sc-42 has been performed at the JYFL IGISOL IV facility in order to determine the change in nuclear mean-square charge radius between the I-pi = 0(+) ground state and the I-pi = 7(+) isomer via the measurement of the Sc-42g,Sc-42m isomer shift. New multi-configurational Dirac-Fock calculations for the atomic mass shift and field shift factors have enabled a recalibration of the charge radii of the Sc42-46 isotopes which were measured previously. While consistent with the treatment of proton-neutron, proton-proton and neutron-neutron pairing on an equal footing, the reduction in size for the isomer is observed to be of a significantly larger magnitude than that expected from both shell-model and ab-initio calculations. The measured nuclear magnetic dipole moment and electric quadruple moment, on the other hand, are in good agreement with simple empirical estimates and shell-model calculations.

S. Willing, K. Schlage, L. Bocklage, M. M. R. Moayed, T. Gurieva, G. Meier, and R. Röhlsberger
Novel Tunnel Magnetoresistive Sensor Functionalities via Oblique-Incidence Deposition
ACS Applied Materials & Interfaces 13, 32343 (2021)

Abstract: Controlling the magnetic properties of ultrathin films remains one of the main challenges to the further development of tunnel magnetoresistive (TMR) device applications. The magnetic response in such devices is mainly governed by extending the primary TMR trilayer with the use of suitable contact materials. The transfer of magnetic anisotropy to ferromagnetic electrodes consisting of CoFeB layers results in a field-dependent TMR response, which is determined by the magnetic properties of the CoFeB as well as the contact materials. We flexibly apply oblique-incidence deposition (OID) to introduce arbitrary intrinsic in-plane anisotropy profiles into the magnetic layers. The OID-induced anisotropy shapes the magnetic response and eliminates the requirement of additional magnetic contact materials. Functional control is achieved via an adjustable shape anisotropy that is selectively tailored for the ultrathin CoFeB layers. This approach circumvents previous limitations on TMR devices and allows for the design of new sensing functionalities, which can be precisely customized to a specific application, even in the high field regime. The resulting sensors maintain the typical TMR signal strength as well as a superb thermal stability of the tunnel junction, revealing a striking advantage in functional TMR design using anisotropic interfacial roughness.

F. Karbstein
Vacuum Birefringence at the Gamma Factory
Annalen der Physik n/a, 2100137 (2021)

Abstract: Abstract The perspectives of studying vacuum birefringence at the Gamma Factory are explored. To this end, the parameter regime which can be reliably analyzed resorting to the leading contribution to the Heisenberg?Euler effective Lagrangian is assessed in detail. It is explicitly shown that?contrary to naive expectations?this approach allows for the accurate theoretical study of quantum vacuum signatures up to fairly large photon energies. The big advantage of this parameter regime is the possibility of studying the phenomenon in experimentally realistic, manifestly inhomogeneous pump and probe field configurations. Thereafter, two specific scenarios giving rise to a vacuum birefringence effect for traversing gamma probe photons are analyzed. In the first scenario the birefringence phenomenon is induced by a quasi-constant static magnetic field. In the second case it is driven by a counter-propagating high-intensity laser field.

W. Eschen, S. Wang, C. Liu, R. Klas, M. Steinert, S. Yulin, H. Meissner, M. Bussmann, T. Pertsch, J. Limpert, and J. Rothhardt
Towards attosecond imaging at the nanoscale using broadband holography-assisted coherent imaging in the extreme ultraviolet
Communications Physics 4, 154 (2021)

Abstract: The inherently broad bandwidth of attosecond pulses conflicts with the coherence requirements of lensless imaging. Here, broadband holography-assisted coherent imaging is demonstrated with a resolution of less than 35 nm. Nanoscale coherent imaging has emerged as an indispensable modality, allowing to surpass the resolution limit given by classical imaging optics. At the same time, attosecond science has experienced enormous progress and has revealed the ultrafast dynamics in complex materials. Combining attosecond temporal resolution of pump-probe experiments with nanometer spatial resolution would allow studying ultrafast dynamics on the smallest spatio-temporal scales but has not been demonstrated yet. To date, the large bandwidth of attosecond pulses poses a major challenge to high-resolution coherent imaging. Here, we present broadband holography-enhanced coherent imaging, which enables the combination of high-resolution coherent imaging with a large spectral bandwidth. By implementing our method at a high harmonic source, we demonstrate a spatial resolution of 34 nm in combination with a spectral bandwidth of 5.5 eV at a central photon energy of 92 eV. The method is single-shot capable and retrieves the spectrum from the measured diffraction pattern.

B. Böning, and S. Fritzsche
Above-threshold ionization driven by Gaussian laser beams: beyond the electric dipole approximation
Journal of Physics B: Atomic, Molecular and Optical Physics 54, 144002 (2021)

Abstract: Strong-field atomic experiments have recently become sensitive to nondipole (magnetic) interactions. In particular, photoelectrons emitted in above-threshold ionization possess a nonzero momentum along the beam axis as a result of the Lorentz force. Here, we show how this longitudinal momentum can be theoretically calculated based on a nondipole strong-field approximation that accounts not only for the temporal but also the spatial dependence of the laser field in the photoelectron continuum. If the driving laser beam is approximated as a plane wave, the theoretical values differ from known experimental results by a constant offset. We demonstrate that this offset can successfully be removed if a realistic Gaussian beam profile is accounted for in the quantum description of ATI. We also discuss the influence of the size of the beam waist in the focus.

J. Gollwitzer, L. Bocklage, R. Röhlsberger, and G. Meier
Connecting Fano Interference and the Jaynes-Cummings Model in Cavity Magnonics
NPJ Quantum Information 7, 114 (2021)

Abstract: We show that Fano interference can be realized in a macroscopic microwave cavity coupled to a spin ensemble at room temperature. Via a formalism developed from the linearized Jaynes-Cummings model of cavity electromagnonics, we show that generalized Fano interference emerges from the photon–magnon interaction at low cooperativity. In this regime, the reflectivity approximates the scattering cross-section derived from the Fano-Anderson model. Although asymmetric lineshapes in this system are often associated with the Fano formalism, we show that whilst Fano interference is actually present, an exact Fano form cannot be achieved from the linear Jaynes-Cummings model. In the Fano model an additional contribution arises, which is attributed to decoherence in other systems, and in this case is due to the resonant nature of the photonic mode. The formalism is experimentally verified and accounts for the asymmetric lineshapes arising from the interaction between magnon and photon channels. As the magnon–photon coupling strength is increased, these channels merge into hybridized magnon–photon modes and the generalized Fano interference picture breaks down. Our results are universally applicable to systems underlying the linearized Jaynes-Cummings Hamiltonian at low cooperativity and connect the microscopic parameters of the quantum optical model to generalized Fano lineshapes.

V. Schuster, V. Hilbert, R. Klas, C. Liu, M. Tschernajew, B. Bernhardt, J. Rothhardt, and J. Limpert
Agile spectral tuning of high order harmonics by interference of two driving pulses
Optics Express 29, 22117 (2021)

Abstract: In this work, the experimental realization of a tunable high photon flux extreme ultraviolet light source is presented. This is enabled by high harmonic generation of two temporally delayed driving pulses with a wavelength of 1030 nm, resulting in a tuning range of 0.8 eV at the 19th harmonic at 22.8 eV. The implemented approach allows for fast tuning of the spectrum, is highly flexible and is scalable towards full spectral coverage at higher photon energies.

V. Schuster, C. Liu, R. Klas, P. Dominguez, J. Rothhardt, J. Limpert, and B. Bernhardt
Ultraviolet dual comb spectroscopy: a roadmap
Optics Express 29, 21859 (2021)

Abstract: Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy structure of matter. This will access the prime triggers of photochemical reactions with unprecedented spectral resolution. In this research article, we discuss the milestones marking the way to the first UV dual comb spectrometer. We present experimental and simulated studies towards UV dual comb spectroscopy, directly applied to planned absorption measurements of formaldehyde (centered at 343 nm, 3.6 eV) and argon (80 nm, 16 eV). This will enable an unparalleled relative resolution of up to 10-9 - with a table-top UV source surpassing any synchrotron-linked spectrometer by at least two and any grating-based UV spectrometer by up to six orders of magnitude.

P.-M. Hillenbrand, K. N. Lyashchenko, S. Hagmann, O. Andreev, D. Banas, E. P. Benis, I. Bondarev, C. Brandau, E. De Filippo, O. Forstner, J. Glorius, R. E. Grisenti, A. Gumberidze, D. L. Guo, M. O. Herdrich, M. Lestinsky, Y. Litvinov, V. Pagano, N. Petridis, M. S. Sanjari, D. Schury, U. Spillmann, S. Trotsenko, M. Vockert, A. B. Voitkiv, G. Weber, and T. Stoehlker
Electron-loss-to-continuum cusp in collisions of U89+ with N-2 and Xe
Physical Review A 104, 012809 (2021)

Abstract: We study the electron-loss-to-continuum (ELC) cusp experimentally and theoretically by comparing the ionization of U89+ projectiles in collisions with N-2 and Xe targets, at a beam energy of 75.91 MeV/u. The coincidence measurement between the singly ionized projectile and the energy of the emitted electron is used to compare the shape of the ELC cusp at weak and strong perturbations. A significant energy shift for the centroid of the electron cusp is observed for the heavy target of Xe as compared to the light target of N-2. Our results provide a stringent test for fully relativistic calculations of double-differential cross sections performed in the first-order approximation and in the continuum-distorted-wave approach.

J. Hofbrucker, B. Böning, A. V. Volotka, and S. Fritzsche
Elliptical dichroism in biharmonic ionization of atoms
Physical Review A 104, 013102 (2021)

Abstract: In multiphoton ionization of atoms, elliptical dichroism may arise in the photoelectron angular distributions due to the interference of the possible ionization pathways. We here consider the interaction of atoms with an elliptically polarized biharmonic $(\omega + 2\omega)$ field which simultaneously allows one- and two-photon ionization of the atoms. The interference between these two ionization pathways introduces contributions to the elliptical dichroism in addition to the dichroism that arises from the two-photon ionization alone. We show that these additional dichroism contributions can lead to a stronger dichroism in comparison to the one arising from two-photon ionization only. We present a relativistic analysis of the corresponding photoelectron angular distributions and discuss individual contributions to the dichroic phenomena. Detailed computations have been performed for biharmonic ionization of neutral helium atoms.

F. Liu, Z. Chen, T. Morishita, K. Bartschat, B. Böning, and S. Fritzsche
Single-cycle versus multicycle nonsequential double ionization of argon
Physical Review A 104, 013105 (2021)

Abstract: Using an improved quantitative rescattering model, we calculate the correlated two-electron momentum distributions (CMDs) for nonsequential double ionization of Ar exposed to intense laser pulses with a wavelength of 790 nm at a peak intensity of 1.0×10¹⁴ W/cm². We analyze the drastic variations in the CMDs that were observed by Kübel et al. [New J. Phys. 16, 033008 (2014)] in the transition from near-single-cycle to multicycle driving laser pulses. Our model reproduces their experimental data well. We also find that the transition from near-single-cycle to multicycle driving laser pulses depends strongly on the details of the pulse envelope. Special attention is paid to the mechanisms responsible for the cross-shaped structure observed experimentally with 4 fs pulses. Our analysis reveals that the cross-shaped structure in the carrier-envelope phase-averaged CMD for near-single-cycle pulses can be attributed to strong backward scattering of the recolliding electron as well as the narrow momentum distributions of the tunnel-ionized electrons compared to those for long pulses. This also explains why the cross-shaped distributions collapse to a rather structureless distribution when the pulse duration is increased to 8 fs.

R. Hollinger, E. Haddad, M. Zapf, V. Shumakova, P. Herrmann, R. Roeder, I. Uschmann, U. Reisloehner, A. Pugzlys, A. Baltuska, F. Legare, M. Zuerch, C. Ronning, C. Spielmann, and D. Kartashov
Role of free-carrier interaction in strong-field excitations in semiconductors
Physical Review B 104, 035203 (2021)

Abstract: The interaction of laser pulses with condensed matter forms the basis of light-wave-driven electronics potentially enabling tera- and petahertz switching rate applications. Carrier control using near- and midinfrared pulses is appealing for integration into existing platforms. Toward this end, a fundamental understanding of the complexity of phenomena concerning sub-band-gap driven semiconductors such as high harmonic generation, carrier excitation due to multiphoton absorption, and interband tunneling as well as carrier-carrier interactions due to strong acceleration in infrared transients is important. Here, stimulated emission from polycrystalline ZnO thin films for pump wavelengths between 1.2 mu m (1 eV) and 10 mu m (0.12 eV) is observed. Contrary to the expected higher intensity threshold for longer wavelengths, the lowest threshold pump intensity for stimulated emission is obtained for the longest pump wavelength corroborating the importance of collisional excitation upon intraband electron acceleration.

E. Mosman, and F. Karbstein
Vacuum birefringence and diffraction at an x-ray free-electron laser: From analytical estimates to optimal parameters
Physical Review D 104, 013006 (2021)

Abstract: We study vacuum birefringence and x-ray photon scattering in the head-on collision of x-ray free electron and high-intensity laser pulses. Resorting to analytical approximations for the numbers of attainable signal photons, we analyze the behavior of the phenomenon under the variation of various experimental key-parameters and provide new analytical scalings. Our optimized approximations allow for quantitatively accurate results on the one-percent level. We in particular demonstrate that an appropriate choice of the x-ray focus and pulse duration can significantly improve the signal for given laser parameters, using the experimental parameters to be available at the Helmholtz International Beamline for Extreme Fields at the European XFEL as example. Our results are essential for the identification of the optimal choice of parameters in a discovery experiment of vacuum birefringence at the high-intensity frontier.

P. Wustelt, F. Oppermann, S. Mhatre, M. Kuebel, A. Sayler, M. Lein, S. Graefe, and G. Paulus
Laser-Driven Anharmonic Oscillator: Ground-State Dissociation of the Helium Hydride Molecular Ion by Midinfrared Pulses
Physical Review Letters 127, 043202 (2021)

Abstract: The vibrational motion of molecules represents a fundamental example of an anharmonic oscillator. Using a prototype molecular system, HeH+, we demonstrate that appropriate laser pulses make it possible to drive the nuclear motion in the anharmonic potential of the electronic ground state, increasing its energy above the potential barrier and facilitating dissociation by purely vibrational excitation. We find excellent agreement between the frequency-dependent response of the helium hydride molecular cation to both classical and quantum mechanical simulations, thus removing any ambiguities through electronic excitation. Our results provide access to the rich dynamics of anharmonic quantum oscillator systems and pave the way to state-selective control schemes in ground-state chemistry by the adequate choice of the laser parameters.

T. Kaaden, V. Tympel, M. Kober, F. Schmidl, M. Rettenmayr, and S. Lippmann
Electric pulse heating device for the analysis of solid/solid phase transformations
Review of Scientific Instruments 92, 074703 (2021)

Abstract: Ohmic pulse heating is applied to investigate diffusion and interface controlled solid-state phase transformations. The developed device uses extensive solid-state electronics providing a high current, low voltage approach that overcomes the limitations of existing setups, most notably the use of sample geometries that allow for the reliable measurement of local temperatures and their assignment to microstructures. Power for heating is supplied by a capacitor array with adjustable voltage, and the process is controlled by microcontrollers and a solid-state relay, which allows for controlled pulses that are adjustable in microseconds. Electric currents of up to 22 kA at 90 V can be realized by the setup. Electric data are monitored and collected during the experiments, and temperature data are captured using a high-resolution infrared camera at high frame rates (1200 fps). The capabilities of the setup are demonstrated by rapid heating (10(6) K/s) and subsequent cooling of a brass sample. Two distinct areas of the sample are analyzed in detail, showing similar heating, but different cooling curves with rates of 10(4) and 10(2) K/s. Local microstructure analysis shows that different phase transformation mechanisms were dominant, and thus, the setup fulfills its purpose.

M. Alamoudi, M. Sattari, M. Balubaid, E. Eftekhari-Zadeh, E. Nazemi, O. Taylan, and E. Kalmoun
Application of Gamma Attenuation Technique and Artificial Intelligence to Detect Scale Thickness in Pipelines in Which Two-Phase Flows with Different Flow Regimes and Void Fractions Exist
Symmetry 13, 1198 (2021)

Abstract: Scale deposits can reduce equipment efficiency in the oil and petrochemical industry. The gamma attenuation technique can be used as a non-invasive effective tool for detecting scale deposits in petroleum pipelines. The goal of this study is to propose a dual-energy gamma attenuation method with radial basis function neural network (RBFNN) to determine scale thickness in petroleum pipelines in which two-phase flows with different symmetrical flow regimes and void fractions exist. The detection system consists of a dual-energy gamma source, with Ba-133 and Cs-137 radioisotopes and two 2.54-cm x 2.54-cm sodium iodide (NaI) detectors to record photons. The first detector related to transmitted photons, and the second one to scattered photons. The transmission detector recorded two signals, which were the counts under photopeak of Ba-133 and Cs-137 with the energy of 356 keV and 662 keV, respectively. The one signal recorded in the scattering detector, total counts, was applied to RBFNN as the inputs, and scale thickness was assigned as the output.

A. Gumberidze, D. Thorn, A. Surzhykov, C. Fontes, D. Banas, H. Beyer, W. Chen, R. Grisenti, S. Hagmann, R. Hess, P.-M. Hillenbrand, P. Indelicato, C. Kozhuharov, M. Lestinsky, R. Märtin, N. Petridis, R. Popov, R. Schuch, U. Spillmann, S. Tashenov, S. Trotsenko, A. Warczak, G. Weber, W. Wen, D. Winters, N. Winters, Z. Yin, and T. Stöhlker
Angular Distribution of Characteristic Radiation Following the Excitation of He-Like Uranium in Relativistic Collisions
Atoms 9, 20 (2021)

Abstract: In this paper, we present an experimental and theoretical study of excitation processes for the heaviest stable helium-like ion, that is, He-like uranium occurring in relativistic collisions with hydrogen and argon targets. In particular, we concentrate on angular distributions of the characteristic K alpha radiation following the K -> L excitation of He-like uranium. We pay special attention to the magnetic sub-level population of the excited 1s2l(j) states, which is directly related to the angular distribution of the characteristic K alpha radiation. We show that the experimental data can be well described by calculations taking into account the excitation by the target nucleus as well as by the target electrons. Moreover, we demonstrate for the first time an important influence of the electron-impact excitation process on the angular distributions of the K alpha radiation produced by excitation of He-like uranium in collisions with different targets.

M. Mueller, J. Buldt, H. Stark, C. Grebing, and J. Limpert
Multipass cell for high-power few-cycle compression
Optics letters 46, 2678 (2021)

Abstract: A multipass cell for nonlinear compression to few-cycle pulse duration is introduced composing dielectrically enhanced silver mirrors on silicon substrates. Spectral broadening with 388 W output average power and 776 mu J pulse energy is obtained at 82% cell transmission. A high output beam quality (M-2 < 1.2) and a high spatio-spectral homogeneity (97.5%), as well as the compressibility of the output pulses to 6.9 fs duration, are demonstrated. A finite element analysis reveals scalability of this cell to 2 kW average output power.

B. Baghdasaryan, F. Steinlechner, and S. Fritzsche
Justifying the thin-crystal approximation in spontaneous parametric down-conversion for collinear phase matching
Physical Review A 103, 063508 (2021)

Abstract: Spatially engineered photons from spontaneous parametric down-conversion (SPDC) are a valuable tool for studying and applying photonic entanglement. An advantage of SPDC is that simple expressions for the two-photon state can be obtained using justified approximations. In particular, the thin-crystal approximation has often been invoked in the engineering of high-dimensional entangled states. Knowledge of the conditions under which the thin-crystal approximation remains valid is essential for the realization of experimental setups. We provide a quantitative guideline on the validity of the thin-crystal approximation in calculating the two-photon spatial state. In particular, we show that the applicability of this regime is related to the focusing parameter (w) over barp = w(p)/root lambda(p) L, where w(p) and lambda(p) are the beam waist and wavelength of the pump beam, respectively, and L is the length of the nonlinear crystal. Additionally, the validity of the thin-crystal regime is investigated concerning the size of a subspace in the Laguerre Gaussian basis, into which the two-photon state can be projected in a given experiment.

G. von Gersdorff, S. Panahiyan, and W. Chen
Unification of topological invariants in Dirac models
Physical Review B 103, 245146 (2021)

Abstract: Topological phases of materials are characterized by topological invariants that are conventionally calculated by different means according to the dimension and symmetry class of the system. For topological materials described by Dirac models, we introduce a wrapping number as a unified approach to obtain the topological invariants in arbitrary dimensions and symmetry classes. Given a unit vector that parametrizes the momentum dependence of the Dirac model, the wrapping number describes the degree of the map from the Brillouin zone torus to the sphere formed by the unit vector that we call the Dirac sphere. This method is gauge-invariant and originates from the intrinsic features of the Dirac model and moreover places all known topological invariants, such as the Chern number, winding number, Pfaffian, etc, on equal footing.

H. Gies, and A. Salek
Curvature bound from gravitational catalysis in thermal backgrounds
Physical Review D 103, 125027 (2021)

Abstract: We investigate the phenomenon of gravitational catalysis, i.e., curvature-induced chiral symmetry breaking and fermion mass generation, at finite temperature. Using a scale-dependent analysis, we derive a thermal bound on the curvature of local patches of spacetime. This bound quantifies regions in parameter space that remain unaffected by gravitational catalysis and thus are compatible with the existence of light fermions as observed in nature. While finite temperature generically relaxes the curvature bound, we observe a comparatively strong dependence of the phenomenon on the details of the curvature. Our bound can be applied to scenarios of quantum gravity, as any realistic candidate has to accommodate a sufficient number of light fermions. We argue that our bound therefore represents a test for quantum-gravity scenarios: A suitably averaged spacetime in the (trans-)Planckian regime that satisfies our curvature bound does not induce correspondingly large Planckian fermion masses by gravitational catalysis. The temperature dependence derived in this work facilitates to follow the fate of gravitational catalysis during the thermal history of the (quantum) Universe. In an application to the asymptotic-safety scenario of quantum gravity, our bound translates into a temperature-dependent upper bound on the number of fermion flavors.

Y. Ma, D. Seipt, K. Krushelnick, and A. G. R. Thomas
Generation of straight and curved hollow plasma channels by laser-generated nonlinear wakefields and studies of ultra-intense laser pulse guiding
Physics of Plasmas 28, 063104 (2021)

Abstract: We report on a study of highly controllable, quasi-static hollow plasma channels generated by ion motion following a laser–plasma interaction via numerical simulations. These channels are generated by ion motion in a nonlinear wakefield, which has an asymmetry between focusing and defocusing periods. Such plasma channels, driven by a fs duration, 100 TW level laser pulse, have the capability to guide more powerful laser pulses. Moreover, we show that curved plasma channels can be generated in a transverse density gradient plasma and all-optical guiding of a second, significantly more powerful laser pulse in such a curved plasma channel. This mechanism may be useful for creating plasma optics for multi-stage TeV laser plasma accelerators and compact synchrotron radiation sources.

Y. Ma, D. Seipt, A. E. Hussein, S. Hakimi, N. F. Beier, S. B. Hansen, J. Hinojosa, A. Maksimchuk, J. Nees, K. Krushelnick, A. G. R. Thomas, and F. Dollar
The effects of laser polarization and wavelength on injection dynamics of a laser wakefield accelerator
Physics of Plasmas 28, 063101 (2021)

Abstract: Here, we investigate the effects of laser polarization and wavelength on electron injection dynamics in a laser wakefield accelerator. During the ionization process, electrons gain residual momentum and kinetic energy via above threshold ionization, which has a strong dependence on laser polarization. A circularly polarized laser pulse results in a much higher residual momentum and kinetic energy gain for the ionized electrons compared with the linearly polarized case. This residual momentum results in particle injection because of the sensitivity of particle trapping to the initial conditions and enhanced the total injected beam charge in both experiments and particle-in-cell simulations. Due to the strong correlation of above threshold ionization with laser wavelength, in this work we extended the investigation to long wavelength (up to 20 μm) drive pulses using particle-in-cell simulations. Owing to the gain in kinetic energy, it may be expected that the charge trapped would consistently increase for circular polarization with increasing laser wavelength, but this was not observed. Instead, there are oscillations with wavelength in the relative trapped charge between linear and circular polarization cases, which arise because of ionization and heating effects on the plasma. Our studies highlight the complex interplay between several different physical effects, including injection regimes—above threshold ionization assisted injection, wave-breaking injection by carrier-envelope-phase effects and ionization injection—ionization gradient induced laser pulse evolution, and thermal modifications to the wake structure that need considering when extrapolating laser wakefield acceleration to different wavelength regimes.

R. Soguel, A. Volotka, D. Glazov, and S. Fritzsche
Many-Electron QED with Redefined Vacuum Approach
Symmetry 13, 1014 (2021)

Abstract: The redefined vacuum approach, which is frequently employed in the many-body perturbation theory, proved to be a powerful tool for formula derivation. Here, we elaborate this approach within the bound-state QED perturbation theory. In addition to general formulation, we consider the particular example of a single particle (electron or vacancy) excitation with respect to the redefined vacuum. Starting with simple one-electron QED diagrams, we deduce first- and second-order many-electron contributions: screened self-energy, screened vacuum polarization, one-photon exchange, and two-photon exchange. The redefined vacuum approach provides a straightforward and streamlined derivation and facilitates its application to any electronic configuration. Moreover, based on the gauge invariance of the one-electron diagrams, we can identify various gauge-invariant subsets within derived many-electron QED contributions.

M. Ruijter, V. Petrillo, T. Teter, M. Valialshchikov, and S. Rykovanov
Signatures of the Carrier Envelope Phase in Nonlinear Thomson Scattering
Crystals 11, 528 (2021)

Abstract: High-energy radiation can be generated by colliding a relativistic electron bunch with a high-intensity laser pulse-a process known as Thomson scattering. In the nonlinear regime the emitted radiation contains harmonics. For a laser pulse whose length is comparable to its wavelength, the carrier envelope phase changes the behavior of the motion of the electron and therefore the radiation spectrum. Here we show theoretically and numerically the dependency of the spectrum on the intensity of the laser and the carrier envelope phase. Additionally, we also discuss what experimental parameters are required to measure the effects for a beamed pulse.

S. Fritzsche, and A. Surzhykov
Approximate Atomic Green Functions
Molecules 26, 2660 (2021)

Abstract: In atomic and many-particle physics, Green functions often occur as propagators to formally represent the (integration over the) complete spectrum of the underlying Hamiltonian. However, while these functions are very crucial to describing many second- and higher-order perturbation processes, they have hardly been considered and classified for complex atoms. Here, we show how relativistic (many-electron) Green functions can be approximated and systematically improved for few- and many-electron atoms and ions. The representation of these functions is based on classes of virtual excitations, or so-called excitation schemes, with regard to given bound-state reference configurations, and by applying a multi-configuration Dirac-Hartree-Fock expansion of all atomic states involved. A first implementation of these approximate Green functions has been realized in the framework of Jac, the Jena Atomic Calculator, and will facilitate the study of various multi-photon and/or multiple electron (emission) processes.

D. Seipt, C. P. Ridgers, D. Del Sorbo, and A. G. R. Thomas
Polarized QED cascades
New Journal of Physics 23, 053025 (2021)

Abstract: By taking the spin and polarization of the electrons, positrons and photons into account in the strong-field QED processes of nonlinear Compton emission and pair production, we find that the growth rate of QED cascades in ultra-intense laser fields can be substantially reduced. While this means that fewer particles are produced, we also found them to be highly polarized. We further find that the high-energy tail of the particle spectra is polarized opposite to that expected from Sokolov–Ternov theory, which cannot be explained by just taking into account spin-asymmetries in the pair production process, but results significantly from ‘spin-straggling’. We employ a kinetic equation approach for the electron, positron and photon distributions, each of them spin/polarization-resolved, with the QED effects of photon emission and pair production modelled by a spin/polarization dependent Boltzmann-type collision operator. For photon-seeded cascades, depending on the photon polarization, we find an excess or a shortage of particle production in the early stages of cascade development, which provides a path towards a controlled experiment. Throughout this paper we focus on rotating electric field configuration, which represent an idealized model and allows for a straightforward interpretation of the observed effects.

C. Gaida, M. Gebhardt, T. Heuermann, Z. Wang, C. Jauregui, and J. Limpert
Transverse mode instability and thermal effects in thulium-doped fiber amplifiers under high thermal loads
Optics Express 29, 14963 (2021)

Abstract: We experimentally analyze the average-power-scaling capabilities of ultrafast, thulium-doped fiber amplifiers. It has been theoretically predicted that thulium-doped fiber laser systems, with an emission wavelength around 2 mu m, should be able to withstand much higher heat-loads than their Yb-doped counterparts before the onset of transverse mode instability (TMI) is observed. In this work we experimentally verify this theoretical prediction by operating thulium doped fibers at very high heat-load. In separate experiments we analyze the performance of two different large-core, thulium-doped fiber amplifiers. The first experiment aims at operating a short, very-large core, thulium-doped fiber amplifier at extreme heat-load levels of more than 300 W/m. Even at this extreme heat-load level, the onset of TMI is not observed. The second experiment maximizes the extractable average-output power from a large-core, thulium-doped, fiber amplifier. We have achieved a pump-limited average output power of 1.15 kW without the onset of TMI. However, during a longer period of operation at this power level the amplifier performance steadily degraded and TMI could be observed for average powers in excess of 847 W thereafter. This is the first time, to the best of our knowledge, that TMI has been reported in a thulium-doped fiber amplifier.

T. Helk, E. Berger, S. Jamnuch, L. Hoffmann, A. Kabacinski, J. Gautier, F. Tissandier, J.-P. Goddet, H.-T. Chang, J. Oh, C. Das Pemmaraju, T. Pascal, S. Sebban, C. Spielmann, and M. Zuerch
Table-top extreme ultraviolet second harmonic generation
Science Advances 7, 2265 (2021)

Abstract: The lack of available table-top extreme ultraviolet (XUV) sources with high enough fluxes and coherence properties has limited the availability of nonlinear XUV and x-ray spectroscopies to free-electron lasers ( FELs). Here, we demonstrate second harmonic generation (SHG) on a table-top XUV source by observing SHG near the TiM2,3 edge with a high-harmonic seeded soft x-ray laser. Furthermore, this experiment represents the first SHG experiment in the XUV. First-principles electronic structure calculations suggest the surface specificity and separate the observed signal into its resonant and nonresonant contributions. The realization of XUV-SHG on a table-top source opens up more accessible opportunities for the study of element-specific dynamics in multicomponent systems where surface, interfacial, and bulk-phase asymmetries play a driving role.

S. Skruszewicz, S. Fuchs, J. J. Abel, J. Nathanael, J. Reinhard, C. Rödel, F. Wiesner, M. Wuensche, P. Wachulak, A. Bartnik, K. Janulewicz, H. Fiedorowicz, and G. G. Paulus
Coherence tomography with broad bandwidth extreme ultraviolet and soft X-ray radiation
Applied Physics B 127, 55 (2021)

Abstract: We present an overview of recent results on optical coherence tomography with the use of extreme ultraviolet and soft X-ray radiation (XCT). XCT is a cross-sectional imaging method that has emerged as a derivative of optical coherence tomography (OCT). In contrast to OCT, which typically uses near-infrared light, XCT utilizes broad bandwidth extreme ultraviolet (XUV) and soft X-ray (SXR) radiation (Fuchs et al in Sci Rep 6:20658, 2016). As in OCT, XCT\textquotesingle s axial resolution only scales with the coherence length of the light source. Thus, an axial resolution down to the nanometer range can be achieved. This is an improvement of up to three orders of magnitude in comparison to OCT. XCT measures the reflected spectrum in a common-path interferometric setup to retrieve the axial structure of nanometer-sized samples. The technique has been demonstrated with broad bandwidth XUV/SXR radiation from synchrotron facilities and recently with compact laboratory-based laser-driven sources. Axial resolutions down to 2.2 nm have been achieved experimentally. XCT has potential applications in three-dimensional imaging of silicon-based semiconductors, lithography masks, and layered structures like XUV mirrors and solar cells.

S. Sadashivaiah, J. Wolny, L. Scherthan, K. Jenni, A. Omlor, C. Mueller, I. Sergueev, M. Herlitschke, O. Leupold, H.-C. Wille, R. Röhlsberger, and V. Schuenemann
High-Repetition Rate Optical Pump-Nuclear Resonance Probe Experiments Identify Transient Molecular Vibrations after Photoexcitation of a Spin Crossover Material
Journal of Physical Chemistry Letters 12, 3240 (2021)

Abstract: Phonon modes play a vital role in the cooperative phenomenon of light-induced spin transitions in spin crossover (SCO) molecular complexes. Although the cooperative vibrations, which occur over several hundreds of picoseconds to nanoseconds after photoexcitation, are understood to play a crucial role in this phase transition, they have not been precisely identified. Therefore, we have performed a novel optical laser pump-nuclear resonance probe experiment to identify the Fe-projected vibrational density of states (pDOS) during the first few nanoseconds after laser excitation of the mononuclear Fe(II) SCO complex [Fe(PM-BiA)(2)(NCS)(2)]. Evaluation of the so obtained nanosecond-resolved pDOS yields an excitation of similar to 8% of the total volume of the complex from the low-spin to high-spin state. Density functional theory calculations allow simulation of the observed changes in the pDOS and thus identification of the transient inter- and intramolecular vibrational modes at nanosecond time scales.